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@ARTICLE{Li:1005593,
author = {Li, Yun and Krämer, Martina and Mahnke, Christoph and
Rohs, Susanne and Bundke, Ulrich and Spelten, Nicole and
Dekoutsidis, Georgios and Gross, Silke and Voigt, Christiane
and Schumann, Ulrich and Petzold, Andreas},
title = {{U}pper-tropospheric slightly ice-subsaturated regions:
frequency of occurrence and statistical evidence for the
appearance of contrail cirrus},
journal = {Atmospheric chemistry and physics},
volume = {23},
number = {3},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {FZJ-2023-01552},
pages = {2251-2271},
year = {2023},
abstract = {Microphysical, optical, and environmental properties of
contrail cirrus and natural cirrus were investigated by
applying a new, statistically based contrail-cirrus
separation method to 14.7 h of cirrus cloud measurements
(sampling frequency 1 Hz, max. similar to 290 m s(-1), total
length of sampled in-cloud space similar to 15 000 km)
during the airborne campaign ML-CIRRUS in central Europe and
the northeast Atlantic flight corridor in spring 2014. We
find that pure contrail cirrus appears frequently at the
aircraft cruising altitude (CA) range with ambient pressure
varying from 200 to 245 hPa. It exhibits a higher median ice
particle number concentration (N-ice), a smaller median mass
mean radius (R-ice), and lower median ice water content
(IWC) (median: Nice=0.045 cm(-3), R-ice=16.6 mu m, IWC = 3.5
ppmv), and it is optically thinner (median extinction
coefficient Ext = similar to 0.056 km(-1)) than the cirrus
mixture of contrail cirrus, natural in situ-origin and
liquid-origin cirrus found around the CA range (median:
N-ice=0.038 cm(-3), R-ice=24.1 mu m, IWC = 8.3 ppmv, Ext
=similar to 0.096 km(-1)). The lowest and thickest cirrus,
consisting of a few large ice particles, are identified as
pure natural liquid-origin cirrus (median: N-ice=0.018
cm(-3), R-ice=42.4 mu m, IWC = 21.7 ppmv, Ext = similar to
0.137 km(-1)). Furthermore, we observe that, in particular,
contrail cirrus occurs more often in slightly
ice-subsaturated instead of merely ice-saturated to
supersaturated air as often assumed, thus indicating the
possibility of enlarged contrail cirrus existence regions.
The enlargement is estimated, based on IAGOS long-term
observations of relative humidity with respect to ice
(RHice) aboard passenger aircraft, to be approximately 10
$\%$ for Europe and the North Atlantic region, with the
RHice threshold for contrail cirrus existence decreased from
100 $\%$ to 90 $\%$ RHice and a 4 h lifetime of contrail
cirrus in slight ice subsaturation assumed. This increase
may not only lead to a non-negligible change in contrail
cirrus coverage and radiative forcing, but also affect the
mitigation strategies of reducing contrails by rerouting
flights.},
cin = {IEK-7 / IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-7-20101013 / I:(DE-Juel1)IEK-8-20101013},
pnm = {2112 - Climate Feedbacks (POF4-211)},
pid = {G:(DE-HGF)POF4-2112},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000938012500001},
doi = {10.5194/acp-23-2251-2023},
url = {https://juser.fz-juelich.de/record/1005593},
}