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001006570 1001_ $$00000-0002-4408-6657$$aUddin, Nasir$$b0
001006570 245__ $$aUltrabroadband plasmon driving selective photoreforming of methanol under ambient conditions
001006570 260__ $$aWashington, DC$$bNational Acad. of Sciences$$c2023
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001006570 520__ $$aPhotoreforming of methanol has been envisioned as a promising pathway to produce H2 fuel which gained interest over the years. However, the formation of CO2/CO byproducts from this pathway has seen as a major hurdle to its practical realization because the evolution of CO2 and/or CO gases will negatively contribute toward the global-warming and/or environmental issues. To resolve these issues, herein, we discovered solar-driven ultrabroadband plasmonic photoreforming of pure methanol to pure, green and self-separable H2 energy production with zero-emission from an all-plasmonic Cu–WC/W catalytic system. The local electric field, lattice misfit strain, and the monodirectional flow of charge carriers by optical dielectric gradient work in synergy to enable the superior plasmonic photocatalysis in this all-plasmonic system.
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001006570 7001_ $$00000-0001-5403-6912$$aSun, Zhehao$$b1
001006570 7001_ $$0P:(DE-HGF)0$$aLangley, Julien$$b2
001006570 7001_ $$0P:(DE-HGF)0$$aLu, Haijao$$b3
001006570 7001_ $$0P:(DE-Juel1)180314$$aCao, Pengfei$$b4$$eCorresponding author
001006570 7001_ $$00000-0002-5631-4872$$aWibowo, Ary$$b5
001006570 7001_ $$0P:(DE-HGF)0$$aYin, Xinmao$$b6
001006570 7001_ $$0P:(DE-HGF)0$$aTang, Chi Sin$$b7
001006570 7001_ $$0P:(DE-HGF)0$$aNguyen, Hieu T.$$b8
001006570 7001_ $$00000-0001-9521-2601$$aEvans, Jack D.$$b9
001006570 7001_ $$00000-0001-6636-0496$$aLi, Xinzhe$$b10
001006570 7001_ $$0P:(DE-HGF)0$$aZhang, Xiaoliang$$b11
001006570 7001_ $$0P:(DE-Juel1)130695$$aHeggen, Marc$$b12
001006570 7001_ $$0P:(DE-Juel1)144121$$aDunin-Borkowski, Rafal E.$$b13
001006570 7001_ $$00000-0002-5828-4312$$aWee, Andrew T. S.$$b14
001006570 7001_ $$0P:(DE-HGF)0$$aZhao, Haitao$$b15
001006570 7001_ $$0P:(DE-HGF)0$$aCox, Nicholas$$b16
001006570 7001_ $$00000-0002-0800-4490$$aYin, Zongyou$$b17
001006570 773__ $$0PERI:(DE-600)1461794-8$$a10.1073/pnas.2212075120$$gVol. 120, no. 3, p. e2212075120$$n3$$pe2212075120$$tProceedings of the National Academy of Sciences of the United States of America$$v120$$x0027-8424$$y2023
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