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001006607 1001_ $$0P:(DE-HGF)0$$aFaraone, Antonio$$b0$$eCorresponding author
001006607 245__ $$aDynamics of the extended and intermediate range order in model polymer electrolyte poly(ethylene oxide) and lithium bis(trifluoromethanesulfonyl)imide
001006607 260__ $$aLausanne$$bFrontiers Media$$c2023
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001006607 520__ $$aThe dynamics of lithium ions and polymer chains were investigated at the molecular scale in the model polymer electrolyte Poly (ethylene oxide) (PEO)/Lithium bis(trifluoromethanesulfonyl)imide as a function of temperature. This system is known to present an intermediate range order from the arrangement of neighboring chain segments as well as an extended range order of cylindrically arranged chains. The collective dynamics of the systems at lengthscales matching these structural features was measured using Neutron Spin Echo spectroscopy, gaining insights into their lifetime. Moreover, using isotope substitution techniques the dynamics of the lithium ions with respect to the other atoms was probed. The obtained results are compared with the conductivity and the lithium self-diffusion coefficient measured by NMR to gain experimental insight on the molecular processes triggering lithium transport.
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001006607 7001_ $$0P:(DE-HGF)0$$aFalus, Peter$$b1
001006607 7001_ $$0P:(DE-Juel1)172658$$aFörster, Stephan$$b2$$ufzj
001006607 7001_ $$0P:(DE-HGF)0$$aHong, Kunlun$$b3
001006607 7001_ $$0P:(DE-Juel1)130872$$aOhl, Michael$$b4$$ufzj
001006607 773__ $$0PERI:(DE-600)3106355-X$$a10.3389/frsfm.2023.1161141$$gVol. 3, p. 1161141$$p1161141$$tFrontiers in soft matter$$v3$$x2813-0499$$y2023
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