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@ARTICLE{Faraone:1006607,
      author       = {Faraone, Antonio and Falus, Peter and Förster, Stephan and
                      Hong, Kunlun and Ohl, Michael},
      title        = {{D}ynamics of the extended and intermediate range order in
                      model polymer electrolyte poly(ethylene oxide) and lithium
                      bis(trifluoromethanesulfonyl)imide},
      journal      = {Frontiers in soft matter},
      volume       = {3},
      issn         = {2813-0499},
      address      = {Lausanne},
      publisher    = {Frontiers Media},
      reportid     = {FZJ-2023-01744},
      pages        = {1161141},
      year         = {2023},
      abstract     = {The dynamics of lithium ions and polymer chains were
                      investigated at the molecular scale in the model polymer
                      electrolyte Poly (ethylene oxide) (PEO)/Lithium
                      bis(trifluoromethanesulfonyl)imide as a function of
                      temperature. This system is known to present an intermediate
                      range order from the arrangement of neighboring chain
                      segments as well as an extended range order of cylindrically
                      arranged chains. The collective dynamics of the systems at
                      lengthscales matching these structural features was measured
                      using Neutron Spin Echo spectroscopy, gaining insights into
                      their lifetime. Moreover, using isotope substitution
                      techniques the dynamics of the lithium ions with respect to
                      the other atoms was probed. The obtained results are
                      compared with the conductivity and the lithium
                      self-diffusion coefficient measured by NMR to gain
                      experimental insight on the molecular processes triggering
                      lithium transport.},
      cin          = {JCNS-1},
      ddc          = {620},
      cid          = {I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {633 - Life Sciences – Building Blocks of Life: Structure
                      and Function (POF4-633) / 6G4 - Jülich Centre for Neutron
                      Research (JCNS) (FZJ) (POF4-6G4)},
      pid          = {G:(DE-HGF)POF4-633 / G:(DE-HGF)POF4-6G4},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.3389/frsfm.2023.1161141},
      url          = {https://juser.fz-juelich.de/record/1006607},
}