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001006630 245__ $$aPolyelectrolyte Complexes from Oppositely Charged Filamentous Viruses
001006630 260__ $$aWashington, DC$$bACS Publ.$$c2023
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001006630 520__ $$aHere, we present an explorative study on a new type of polyelectrolyte complex made from chemically modified filamentous fd viruses. The fd virus is a semiflexible rod-shaped bacteriophage with a length of 880 nm and a diameter of 6.6 nm, which has been widely used as a well-defined model system of colloidal rods to investigate phase, flow, and other behavior. Here, chemically modified viruses have been prepared to obtain two types with opposite electrical charges in addition to a steric stabilization layer by poly(ethylene glycol) (PEG) grafting. The complex formation of stoichiometric mixtures of these oppositely charged viruses is studied as a function of virus and salt concentration. Furthermore, static light scattering measurements show a varying, strong increase in scattering intensity in some samples without visual macroscopic complex formation. Finally, the results of the complex formation are rationalized by comparing to model calculations on the pair interaction potential between oppositely charged viruses.
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001006630 7001_ $$0P:(DE-Juel1)130577$$aBuitenhuis, Johan$$b1$$eCorresponding author
001006630 773__ $$0PERI:(DE-600)2005937-1$$a10.1021/acs.langmuir.2c02790$$gVol. 39, no. 13, p. 4545 - 4556$$n13$$p4545 - 4556$$tLangmuir$$v39$$x0743-7463$$y2023
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