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@ARTICLE{Ye:1006631,
author = {Ye, Ruijie and Ihrig, Martin and Figgemeier, Egbert and
Fattakhova-Rohlfing, Dina and Finsterbusch, Martin},
title = {{A}queous {P}rocessing of {L}i{C}o{O} 2 –{L}i 6.6 {L}a 3
{Z}r 1.6 {T}a 0.4 {O} 12 {C}omposite {C}athode for
{H}igh-{C}apacity {S}olid-{S}tate {L}ithium {B}atteries},
journal = {ACS sustainable chemistry $\&$ engineering},
volume = {11},
number = {13},
issn = {2168-0485},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {FZJ-2023-01764},
pages = {5184 - 5194},
year = {2023},
abstract = {To fabricate ceramic composite cathodes
LiCoO2–Li6.6La3Zr1.6Ta0.4O12 (LCO-LLZTO) on an industrial
scale, a water-based tape-casting process was developed,
which is scalable and environmentally friendly.
Additionally, the cosintering behavior of the two materials,
often leading to poor electrochemical performance, was
optimized via a Li2O-rich atmosphere. The resulting dense,
free-standing, and phase-pure LCO-LLZTO mixed cathodes were
assembled into full cells using a dual-layer solid
polymer-ceramic separator and an In–Li anode. These cells
show very high utilization rates for LCO of approximately
$90\%$ at a high areal capacity of over 3 mAh cm–2,
demonstrating the potential of water-based tape-casting for
a scalable and sustainable manufacturing of oxide-ceramic
based solid-state Li batteries.},
cin = {IEK-1 / IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-12-20141217},
pnm = {1222 - Components and Cells (POF4-122)},
pid = {G:(DE-HGF)POF4-1222},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000951735700001},
doi = {10.1021/acssuschemeng.2c07556},
url = {https://juser.fz-juelich.de/record/1006631},
}