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@ARTICLE{Wang:1007371,
author = {Wang, Kai and Spatschek, Robert},
title = {{P}hase {F}ield {S}tudy of {C}r-{O}xide {G}rowth {K}inetics
in the {C}rofer 22 {APU} {A}lloy {S}upported by {W}agner’s
{T}heory},
journal = {Energies},
volume = {16},
number = {8},
issn = {1996-1073},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2023-02036},
pages = {3574 -},
year = {2023},
abstract = {The Crofer 22 APU alloy is a frequently used metallic
material to manufacture interconnects in solid oxide fuel
cells. However, the formation and evaporation of Cr2O3 not
only increases the electrical resistance but also leads to
the Cr-related degradation over the service time. In order
to investigate the growth kinetics of Cr-oxide, i.e., Cr2O3,
the multi-phase field model coupled with reliable CALPHAD
databases is employed. The phase field simulation results
are benchmarked with the predictions of Wagner’s theory.
Moreover, we evidence the influence of the temperature and
Cr concentration on the ferritic matrix phase and the oxygen
concentration at the Cr2O3/gas interface on the growth
kinetics of Cr-oxide, paving the way for further
investigations of Cr-related solid oxide fuel cell
degradation processes.},
cin = {IEK-2 / JARA-ENERGY},
ddc = {620},
cid = {I:(DE-Juel1)IEK-2-20101013 / $I:(DE-82)080011_20140620$},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) /
Verbundvorhaben $SOC-Degradation_2$ ' Teilvorhaben A
(03SF0621A) / DFG project 491111487 -
Open-Access-Publikationskosten / 2022 - 2024 /
Forschungszentrum Jülich (OAPKFZJ) (491111487)},
pid = {G:(DE-HGF)POF4-1231 / G:(BMBF)03SF0621A /
G:(GEPRIS)491111487},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000980881100001},
doi = {10.3390/en16083574},
url = {https://juser.fz-juelich.de/record/1007371},
}