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@INPROCEEDINGS{Tober:1007709,
author = {Tober, Steffen and Creutzburg, Marcus and Arndt, Björn and
Chung, Simon and Jacobse, Leon and Jeromin, Arno and Vonk,
Vedran and Stierle, Andreas},
title = {{M}agnetite ({F}e3−𝛿{O}4) homoepitaxy observed by
{X}-ray intensity growth oscillations},
reportid = {FZJ-2023-02175},
year = {2023},
abstract = {Processes on the Fe3−𝛿O4 (001) surface like oxidative
regrowth, (partial)lifting of the subsurface cation vacancy
reconstruction and theelement-specific incorporation of
adatoms demonstrate the sensitiverelation of oxygen
pressure, cation transport and structure in the
nearsurfaceregion of Fe3−𝛿O4 influencing the
performance of catalysts anddevices [1,2,3]. We exemplarily
studied the homoepitaxial growth ofFe3−𝛿O4 (001) in
dependence of the O2 pressure and iron flux. Xrayintensity
growth oscillations proved ordered growth of Fe3−𝛿O4for
all probed conditions while atomic force microscopy revealed
newlyformed micrometre-sized surface structures exceeding
the amount ofdeposited material [4]. Our results indicate
the presence of multipleparallel processes during reactive
Fe3−𝛿O4 homoepitaxy suggestingsimilar processes to
occur also in other applications of Fe3−𝛿O4.[1] Nie et
al., J. Am. Chem. Soc. 135, 10091 (2013), [2] Arndt, B.
etal. PCCP 22, 8336 (2020), [3] Mirabella et al.,
Electrochimica Acta,389, 138638 (2021), [4] van der Vegt et
al., Phys. Rev. Lett. 68, 3335(1992)},
month = {Mar},
date = {2023-03-26},
organization = {DPG-Frühjahrstagung der Sektion
Kondensierte Materie (SKM), Dresden
(Germany), 26 Mar 2023 - 31 Mar 2023},
subtyp = {Invited},
cin = {JCNS-2 / PGI-4 / JARA-FIT},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (FZJ) (POF4-6G4)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G4},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/1007709},
}