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@ARTICLE{Vijayakumar:1008641,
author = {Vijayakumar, Vidyanand and Ghosh, Meena and Asokan, Kiran
and Sukumaran, Santhosh Babu and Kurungot, Sreekumar and
Mindemark, Jonas and Brandell, Daniel and Winter, Martin and
Nair, Jijeesh},
title = {2{D} {L}ayered {N}anomaterials as {F}illers in {P}olymer
{C}omposite {E}lectrolytes for {L}ithium {B}atteries},
journal = {Advanced energy materials},
volume = {13},
number = {15},
issn = {1614-6832},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2023-02442},
pages = {2203326},
year = {2023},
abstract = {Polymer composite electrolytes (PCEs), i.e., materials
combining the disciplines of polymer chemistry, inorganic
chemistry, and electrochemistry, have received tremendous
attention within academia and industry for lithium-based
battery applications. While PCEs often comprise 3D micro- or
nanoparticles, this review thoroughly summarizes the
prospects of 2D layered inorganic, organic, and hybrid
nanomaterials as active (ion conductive) or passive (nonion
conductive) fillers in PCEs. The synthetic inorganic
nanofillers covered here include graphene oxide, boron
nitride, transition metal chalcogenides, phosphorene, and
MXenes. Furthermore, the use of naturally occurring 2D
layered clay minerals, such as layered double hydroxides and
silicates, in PCEs is also thoroughly detailed considering
their impact on battery cell performance. Despite the
dominance of 2D layered inorganic materials, their organic
and hybrid counterparts, such as 2D covalent organic
frameworks and 2D metal–organic frameworks are also
identified as tuneable nanofillers for use in PCE. Hence,
this review gives an overview of the plethora of options
available for the selective development of both the 2D
layered nanofillers and resulting PCEs, which can
revolutionize the field of polymer-based solid-state
electrolytes and their implementation in lithium and
post-lithium batteries.},
cin = {IEK-12},
ddc = {050},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122) / BenchBatt -
Benchmarking und Evaluation der Leistungsfähigkeit und
Kosten von Hochenergie- und Hochvolt-Lithium-Ionen Batterien
im Vergleich zu Post-Lithium-Ionen Technologien (03XP0047B)
/ FestBatt-Polymere - Materialplattform 'Polymere' im Rahmen
des Kompetenzclusters für Festkörperbatterien (13XP0175A)},
pid = {G:(DE-HGF)POF4-1221 / G:(BMBF)03XP0047B /
G:(BMBF)13XP0175A},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000947031300001},
doi = {10.1002/aenm.202203326},
url = {https://juser.fz-juelich.de/record/1008641},
}