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024 7 _ |a 10.1103/PhysRevResearch.5.023157
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100 1 _ |a Kumar, Vivek
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245 _ _ |a Low-temperature antiferromagnetic order in orthorhombic CePdAl 3
260 _ _ |a College Park, MD
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520 _ _ |a We report the magnetization, ac susceptibility, and specific heat of optically float-zoned single crystals of CePdAl3. In comparison to the properties of polycrystalline CePdAl3 reported in the literature, which displays a tetragonal crystal structure and no long-range magnetic order, our single crystals exhibit an orthorhombic structure (Cmcm) and antiferromagnetic order below a Néel temperature T1=5.6 K. The specific heat at zero field shows two anomalies, namely, a broad transition at T1=5.6 K followed by a λ-anomaly at T2=5.4 K. A conservative estimate of the Sommerfeld coefficient of the electronic specific heat, γ=121mJK−2mol−1, indicates a moderately enhanced heavy-fermion ground state. A twin microstructure evolves in the family of planes spanned by the basal plane lattice vectors ao and co , with the magnetic hard axis bo common to all twins. The antiferromagnetic state is characterized by a strong ao, co easy-plane magnetic anisotropy where the ao direction is the easy axis in the easy plane. A spin-flop transition induced under magnetic field along the easy directions, results in complex magnetic phase diagrams. Taken together, our results reveal a high sensitivity of the magnetic and electronic properties of CePdAl3 to its structural modifications.
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700 1 _ |a Bauer, Andreas
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700 1 _ |a Franz, Christian
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700 1 _ |a Spallek, Jan
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700 1 _ |a Schönmann, Rudolf
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700 1 _ |a Stekiel, Michal
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700 1 _ |a Wilde, Marc A.
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700 1 _ |a Pfleiderer, C.
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773 _ _ |a 10.1103/PhysRevResearch.5.023157
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