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@ARTICLE{Shi:1009390,
author = {Shi, Junli and Nguyen, Huu-Dat and Chen, Zhen and Wang, Rui
and Steinle, Dominik and Barnsley, Lester and Li, Jie and
Frielinghaus, Henrich and Bresser, Dominic and Iojoiu,
Cristina and Paillard, Elie},
title = {{N}anostructured block copolymer single-ion conductors for
low-temperature, high-voltage and fast charging
lithium-metal batteries},
journal = {Energy Materials},
volume = {3},
number = {4},
issn = {2770-5900},
address = {Alhambra CA},
publisher = {[Verlag nicht ermittelbar]},
reportid = {FZJ-2023-02794},
pages = {30036},
year = {2023},
abstract = {Herein, a single-ion polymer electrolyte is reported for
high-voltage and low-temperature lithium-metal batteries
that enables suppressing the growth of dendrites, even at
high current densities of 2 mA cm-2. The nanostructured
electrolyte was introduced into the cell by mechanically
processing the polymer powder via an easily scalable
process. Important for the potential application in
commercial battery cells is the finding that it does not
induce aluminum corrosion at high voltages and leads to low
interfacial resistance with lithium metal. These beneficial
characteristics, in combination with its high single-ion
conductivity and its high anodic stability, allow for the
stable cycling of state-of-the-art lithium-ion cathodes,
such as NMC111 and NMC622, in combination with a lithium
metal anode at 20 °C and even 0 °C for several hundred
cycles.},
cin = {JCNS-FRM-II / JCNS-4 / MLZ},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-4-20201012 / I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)KWS1-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001062947500004},
doi = {10.20517/energymater.2023.27},
url = {https://juser.fz-juelich.de/record/1009390},
}