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000010121 0247_ $$2DOI$$a10.1016/j.memsci.2010.04.012
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000010121 084__ $$2WoS$$aEngineering, Chemical
000010121 084__ $$2WoS$$aPolymer Science
000010121 1001_ $$0P:(DE-Juel1)129600$$aCzyperek, M.$$b0$$uFZJ
000010121 245__ $$aGas separation membranes for zero-emission fossil power plants: MEM-BRAIN
000010121 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2010
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000010121 440_0 $$03536$$aJournal of Membrane Science$$v359$$x0376-7388$$y1
000010121 500__ $$aFinancial support from the Helmholtz Association of German Research Centres (Initiative and Networking Fund) through the MEM-BRAIN Helmholtz Alliance is gratefully acknowledged.
000010121 520__ $$aThe objective of the "MEM-BRAIN" project is the development and integration of ceramic and polymeric gas separation membranes for zero-emission fossil power plants. This will be achieved using membranes with a high permeability and selectivity for either CO2, O-2 or H-2, for the three CO2 capture process routes in power plants, thus enabling CO2 to be captured with high-purity in a readily condensable form. For the pre-combustion process, we have developed ceramic microporous membranes that operate at intermediate temperatures (<= 400 degrees C) for H-2/CO2 separation. For the oxyfuel process, we have developed dense ceramic mixed oxygen ionic-electronic conducting membranes that operate at 800-1000 degrees C for O-2/N-2 separation. The perovskite-type oxide Ba0.5Sr0.5Co0.8Fe0.2O3-delta (BSCF5582) was taken as the reference material for this application. For the post-combustion process, polymeric and organic/inorganic hybrid membranes have been developed for CO2/N-2 separation at temperatures up to 200 degrees C. In addition to the development of membranes, we consider the integration of the membranes into power plants by modelling and optimization. Finally, specific technical, economic and environmental properties of CO2 capture as a component in a CCS process chain are assessed, analysing the energy supply system as a whole. (C) 2010 Elsevier B.V. All rights reserved.
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000010121 65320 $$2Author$$aZero-emission power plants
000010121 65320 $$2Author$$aGas separation
000010121 65320 $$2Author$$aCeramic membrane
000010121 65320 $$2Author$$aPolymeric membrane
000010121 65320 $$2Author$$aProcess engineering
000010121 65320 $$2Author$$aSystem integration
000010121 65320 $$2Author$$aEnergy systems analysis
000010121 7001_ $$0P:(DE-Juel1)VDB5094$$aZapp, P.$$b1$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)VDB12702$$aBouwmeester, H. J. M.$$b2$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)VDB92818$$aModigell, M.$$b3$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)VDB21496$$aEbert, K.$$b4$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)VDB92819$$aVoigt, I.$$b5$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)129637$$aMeulenberg, W. A.$$b6$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)129795$$aSingheiser, L.$$b7$$uFZJ
000010121 7001_ $$0P:(DE-Juel1)129666$$aStöver, D.$$b8$$uFZJ
000010121 773__ $$0PERI:(DE-600)1491419-0$$a10.1016/j.memsci.2010.04.012$$gVol. 359$$q359$$tJournal of membrane science$$v359$$x0376-7388$$y2010
000010121 8567_ $$uhttp://dx.doi.org/10.1016/j.memsci.2010.04.012
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