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001014223 1001_ $$0P:(DE-Juel1)179099$$aBuvalaia, Ekaterina$$b0$$ufzj
001014223 245__ $$aInterchain Hydrodynamic Interaction and Internal Friction of Polyelectrolytes
001014223 260__ $$aWashington, DC$$bACS$$c2023
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001014223 520__ $$aPolyelectrolytes (PE) are polymeric macromolecules in aqueous solutions characterized by their chain topology and intrinsic charge in a neutralizing fluid. Structure and dynamics are related to several characteristic screening length scales determined by electrostatic, excluded volume, and hydrodynamic interactions. We examine PE dynamics in dilute to semidilute conditions using dynamic light scattering, neutron spinecho spectroscopy, and pulse field gradient NMR spectroscopy. We connect macroscopic diffusion to segmental chain dynamics, revealing a decoupling of local chain dynamics from interchain interactions. Collective diffusion is described within a colloidal picture, including electrostatic and hydrodynamic interactions. Chain dynamics is characterized by the classical Zimm model of a neutral chain retarded by internal friction. We observe that hydrodynamic interactions are not fully screened between chains and that the internal friction within the chain increases with an increase in ion condensation on the chain.
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001014223 65017 $$0V:(DE-MLZ)GC-1602-2016$$2V:(DE-HGF)$$aPolymers, Soft Nano Particles and  Proteins$$x0
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001014223 7001_ $$0P:(DE-Juel1)130777$$aKruteva, Margarita$$b1
001014223 7001_ $$00000-0001-7178-6467$$aHoffmann, Ingo$$b2
001014223 7001_ $$0P:(DE-Juel1)130905$$aRadulescu, Aurel$$b3$$ufzj
001014223 7001_ $$0P:(DE-Juel1)172658$$aFörster, Stephan$$b4
001014223 7001_ $$0P:(DE-Juel1)130542$$aBiehl, Ralf$$b5$$eCorresponding author
001014223 773__ $$0PERI:(DE-600)2644375-2$$a10.1021/acsmacrolett.3c00409$$gp. 1218 - 1223$$n9$$p1218 - 1223$$tACS Macro Letters$$v12$$x2161-1653$$y2023
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