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001014797 1001_ $$0P:(DE-Juel1)189092$$aJuckel, Martin$$b0$$eCorresponding author$$ufzj
001014797 245__ $$aNovel air-electrode materials for low-cost inert-supported solid oxide cells: investigation of materials compatibility during co-sintering
001014797 260__ $$aDordrecht [u.a.]$$bSpringer Science + Business Media B.V$$c2023
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001014797 520__ $$aFor the investigation of the reactivity of alternative solid oxide cell air electrode materials with forsterite (Mg2SiO4), a magnesium silicate doped with Zn and Ca, five different phase materials were chosen: two Ruddlesden–Popper phase materials: La4Ni3O10 (L4N3) and La3Ni2O7 (L3N2) and three titanium-based perovskite materials: SrTiO3 (STO), SrTi0.75Fe0.25O3 (STF25) and CaTi0.9Fe0.1O3 (CTF). Forsterite was chosen as a support material for the fuel cell, as it is abundant and therefore relatively inexpensive. For the investigation of their reactivity, different types of samples were prepared: mixed pellets, double-layered pellets and screen-printed electrode inks on forsterite green substrates, which were subsequently co-sintered at T = 1300 °C. These samples and their cross sections were then studied using XRD, SEM, EDS and TEM lamella point analysis. Consequently, the impedance spectra were acquired to determine their electro-catalytic performance. The two Ruddlesden–Popper phase materials L4N3 and L3N2 are of high interest due to their thermodynamic stability and high electro-catalytic activity, resulting in a very low polarization resistance. However, this polarization resistance is increased when mixing with forsterite material. In case of the three titanium-based perovskites, the electro-catalytic activity is of less interest due to high polarization resistances.
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001014797 7001_ $$0P:(DE-Juel1)171661$$aGrimm, Fabian$$b1
001014797 7001_ $$0P:(DE-HGF)0$$aZischke, S.$$b2
001014797 7001_ $$0P:(DE-Juel1)159368$$aSohn, Yoo Jung$$b3$$ufzj
001014797 7001_ $$0P:(DE-Juel1)162228$$aGuillon, Olivier$$b4$$ufzj
001014797 7001_ $$0P:(DE-Juel1)129636$$aMenzler, Norbert H.$$b5$$ufzj
001014797 773__ $$0PERI:(DE-600)2015305-3$$a10.1007/s10853-023-08862-0$$gVol. 58, no. 34, p. 13705 - 13720$$n34$$p13705 - 13720$$tJournal of materials science$$v58$$x0022-2461$$y2023
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