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@ARTICLE{Macorano:1014978,
author = {Macorano, Luis and Binny, Taniya M. and Spiegl, Tobias and
Klimenko, Victoria and Singer, Anna and Oberleitner, Linda
and Applegate, Violetta and Seyffert, Sarah and Stefanski,
Anja and Gremer, Lothar and Gertzen, Christoph G. W. and
Höppner, Astrid and Smits, Sander H. J. and Nowack, Eva C.
M.},
title = {{DNA}-binding and protein structure of nuclear factors
likely acting in genetic information processing in the
{P}aulinella chromatophore},
journal = {Proceedings of the National Academy of Sciences of the
United States of America},
volume = {120},
number = {27},
issn = {0027-8424},
address = {Washington, DC},
publisher = {National Acad. of Sciences},
reportid = {FZJ-2023-03522},
pages = {e2221595120},
year = {2023},
abstract = {The chromatophores in Paulinella are
evolutionary-early-stage photosynthetic organelles.
Biological processes in chromatophores depend on a
combination of chromatophore and nucleus-encoded proteins.
Interestingly, besides proteins carrying
chromatophore-targeting signals, a large arsenal of short
chromatophore-targeted proteins (sCTPs; <90 amino acids)
without recognizable targeting signals were found in
chromatophores. This situation resembles endosymbionts in
plants and insects that are manipulated by host-derived
antimicrobial peptides. Previously, we identified an
expanded family of sCTPs of unknown function, named here
"DNA-binding (DB)-sCTPs". DB-sCTPs contain a ~45 amino acid
motif that is conserved in some bacterial proteins with
predicted functions in DNA processing. Here, we explored
antimicrobial activity, DNA-binding capacity, and structures
of three purified recombinant DB-sCTPs. All three proteins
exhibited antimicrobial activity against bacteria involving
membrane permeabilization, and bound to bacterial lipids in
vitro. A combination of in vitro assays demonstrated binding
of recombinant DB-sCTPs to chromatophore-derived genomic DNA
sequences with an affinity in the low nM range.
Additionally, we report the 1.2 Å crystal structure of one
DB-sCTP. In silico docking studies suggest that helix α2
inserts into the DNA major grove and the exposed residues,
that are highly variable between different DB-sCTPs, confer
interaction with the DNA bases. Identification of
photosystem II subunit CP43 as a potential interaction
partner of one DB-sCTP, suggests DB-sCTPs to be involved in
more complex regulatory mechanisms. We hypothesize that
membrane binding of DB-sCTPs is related to their import into
chromatophores. Once inside, they interact with the
chromatophore genome potentially providing nuclear control
over genetic information processing.},
cin = {IBI-7},
ddc = {500},
cid = {I:(DE-Juel1)IBI-7-20200312},
pnm = {5241 - Molecular Information Processing in Cellular Systems
(POF4-524) / SFB 1208 B09 - Erforschung der Kontaktzone
zwischen Wirtszelle und ihren neu erworbenen
photosynthetischen Organellen in der Amöbe Paulinella
chromatophora (Rhizaria, Cercozoa) (B09) (289580405)},
pid = {G:(DE-HGF)POF4-5241 / G:(GEPRIS)289580405},
typ = {PUB:(DE-HGF)16},
pubmed = {37364116},
UT = {WOS:001041172600005},
doi = {10.1073/pnas.2221595120},
url = {https://juser.fz-juelich.de/record/1014978},
}