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@INPROCEEDINGS{Zeng:1015284,
author = {Zeng, Yuan and Schäfer, Laura-Alena and Guillon, Olivier
and Ivanova, Mariya and Leonard, Kwati and Matsumoto,
Hiroshige and Menzler, Norbert H.},
title = {{T}ailoring {P}roperties of {B}a{Z}r0.8-x{C}e0.2{Y}x{O}3-δ
{P}roton {C}onductors for {E}nhanced {P}erformance in
{E}lectrochemical {D}evices},
reportid = {FZJ-2023-03639},
year = {2023},
abstract = {Abstract: In this work, 20 $mol.\%$ of Ce was introduced
into the lattice of Y-doped BaZrO3, and 0.5 $wt.\%$ of NiO
was applied as a sintering aid. The Y2O3 substituent amount
varies within the range of 10-30 $mol.\%$ in order to study
the influence of Y on the phase formation, microstructure,
hydration behavior, electrical performance, mechanical
properties and thermo-chemical stability. The samples were
prepared by solid state reaction combined with traditional
sintering process at 1500 °C for 10h. Y-riched phase has
been found in samples with Y content exceeding 20 $mol.\%.$
Excessive Y2O3 substitution has a negative impact on the
grain boundary conductivity. The grain conductivity
increases linearly with the increase in Y content (except
for the sample with 30 $mol.\%.$ of Y). The impact of Y on
proton conduction in the grain is revealed by integrating
experimental and simulation results. This work provides
comprehensive guidance for the selection of electrolyte
composition for electrochemical devices.Acknowledgement:
Chinese Scholarship Council (CSC); HGF Research Program
“Materials and Technologies for the Energy Transition”
(MTET) - Topic 3: Chemical Energy Carriers.},
month = {Sep},
date = {2023-09-17},
organization = {21st International Conference on
Solid-State Protonic Conductors,
Fukuoka (Japan), 17 Sep 2023 - 22 Sep
2023},
subtyp = {After Call},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)24},
url = {https://juser.fz-juelich.de/record/1015284},
}