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| 001 | 1015304 | ||
| 005 | 20250129094255.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.108.L060403 |2 doi |
| 024 | 7 | _ | |a 2469-9950 |2 ISSN |
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| 100 | 1 | _ | |a Ghosh, Anudeepa |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Anisotropic magnetodielectric coupling in layered antiferromagnetic FePS 3 |
| 260 | _ | _ | |a Woodbury, NY |c 2023 |b Inst. |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a We report anisotropic magnetodielectric coupling in layered van der Waals antiferromagnetic FePS3 (Néel temperature TN∼ 120 K) with perpendicular anisotropy. Above TN, while the dielectric response function along the c axis shows frequency-dependent relaxations, in-plane data is frequency independent and reveals a deviation from phonon-anharmonicity in the ordered state, thereby implying a connection to spin-phonon coupling known to be indicative of onset of magnetic ordering. At low temperature (below 40 K), atypical anomaly in the dielectric constant is corroborated with temperature-dependent dc and ac susceptibility. The magnetodielectric response across this anomaly differs significantly for both in-plane and out-of-plane cases. We have explained this in terms of preferential orientation of magnetic antiferromagnetic zigzag alignment, implied by the in-plane structural anisotropy as confirmed by ab initio calculations. Controlling the relative strength of magnetodielectric coupling with magnetic anisotropy opens a strategy for tracking subtle modifications of structures, such as in-plane anisotropy, with potential applications for spintronic technologies. |
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| 700 | 1 | _ | |a Birowska, Magdalena |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Ghose, Pradeepta Kumar |0 P:(DE-HGF)0 |b 2 |
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| 700 | 1 | _ | |a Bera, Satyabrata |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Bhardwaj, Suresh |0 0000-0002-0716-1267 |b 9 |
| 700 | 1 | _ | |a Nandi, Shibabrata |0 P:(DE-Juel1)177779 |b 10 |
| 700 | 1 | _ | |a Datta, Subhadeep |0 0000-0002-2611-954X |b 11 |e Corresponding author |
| 773 | _ | _ | |a 10.1103/PhysRevB.108.L060403 |g Vol. 108, no. 6, p. L060403 |0 PERI:(DE-600)2844160-6 |n 6 |p L060403 |t Physical review / B |v 108 |y 2023 |x 2469-9950 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/1015304/files/PhysRevB.108.L060403.pdf |y OpenAccess |
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