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001016517 1001_ $$0P:(DE-HGF)0$$aJugovac, Matteo$$b0$$eCorresponding author
001016517 245__ $$aInducing Single Spin‐Polarized Flat Bands in Monolayer Graphene
001016517 260__ $$aWeinheim$$bWiley-VCH$$c2023
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001016517 520__ $$aDue to the fundamental and technological implications in driving the appearance of non-trivial, exotic topological spin textures and emerging symmetry-broken phases, flat electronic bands in 2D materials, including graphene, are nowadays a relevant topic in the field of spintronics. Here, via europium doping, single spin-polarized bands are generated in monolayer graphene supported by the Co(0001) surface. The doping is controlled by Eu positioning, allowing for the formation of a-valley localized single spin-polarized low-dispersive parabolic band close to the Fermi energy when Eu is on top, and of a π* flat band with single spin character when Eu is intercalated underneath graphene. In the latter case, Eu also induces a bandgap opening at the Dirac point while the Eu 4f states act as a spin filter, splitting the π band into two spin-polarized branches. The generation of flat bands with single spin character, as revealed by the spin- and angle-resolved photoemission spectroscopy (ARPES) experiments, complemented by density functional theory (DFT) calculations, opens up new pathways toward the realization of spintronic devices exploiting such novel exotic electronic and magnetic states.
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001016517 7001_ $$0P:(DE-Juel1)176932$$aCojocariu, Iulia$$b1$$ufzj
001016517 7001_ $$0P:(DE-HGF)0$$aSánchez-Barriga, Jaime$$b2
001016517 7001_ $$0P:(DE-HGF)0$$aGargiani, Pierluigi$$b3
001016517 7001_ $$0P:(DE-HGF)0$$aValvidares, Manuel$$b4
001016517 7001_ $$0P:(DE-Juel1)145012$$aFeyer, Vitaliy$$b5
001016517 7001_ $$0P:(DE-Juel1)130548$$aBlügel, Stefan$$b6
001016517 7001_ $$0P:(DE-Juel1)130545$$aBihlmayer, Gustav$$b7
001016517 7001_ $$0P:(DE-HGF)0$$aPerna, Paolo$$b8$$eCorresponding author
001016517 773__ $$0PERI:(DE-600)1474949-X$$a10.1002/adma.202301441$$gVol. 35, no. 38, p. 2301441$$n38$$p2301441$$tAdvanced materials$$v35$$x0935-9648$$y2023
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