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024 7 _ |a 10.1002/adma.202301441
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100 1 _ |a Jugovac, Matteo
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245 _ _ |a Inducing Single Spin‐Polarized Flat Bands in Monolayer Graphene
260 _ _ |a Weinheim
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520 _ _ |a Due to the fundamental and technological implications in driving the appearance of non-trivial, exotic topological spin textures and emerging symmetry-broken phases, flat electronic bands in 2D materials, including graphene, are nowadays a relevant topic in the field of spintronics. Here, via europium doping, single spin-polarized bands are generated in monolayer graphene supported by the Co(0001) surface. The doping is controlled by Eu positioning, allowing for the formation of a-valley localized single spin-polarized low-dispersive parabolic band close to the Fermi energy when Eu is on top, and of a π* flat band with single spin character when Eu is intercalated underneath graphene. In the latter case, Eu also induces a bandgap opening at the Dirac point while the Eu 4f states act as a spin filter, splitting the π band into two spin-polarized branches. The generation of flat bands with single spin character, as revealed by the spin- and angle-resolved photoemission spectroscopy (ARPES) experiments, complemented by density functional theory (DFT) calculations, opens up new pathways toward the realization of spintronic devices exploiting such novel exotic electronic and magnetic states.
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536 _ _ |a SFB 1238 C01 - Strukturinversionsasymmetrische Materie und Spin-Orbit-Phänomene mittels ab initio (C01) (319898210)
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700 1 _ |a Cojocariu, Iulia
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700 1 _ |a Sánchez-Barriga, Jaime
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700 1 _ |a Gargiani, Pierluigi
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700 1 _ |a Valvidares, Manuel
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700 1 _ |a Feyer, Vitaliy
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700 1 _ |a Blügel, Stefan
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700 1 _ |a Bihlmayer, Gustav
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700 1 _ |a Perna, Paolo
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773 _ _ |a 10.1002/adma.202301441
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856 4 _ |u https://juser.fz-juelich.de/record/1016517/files/Advanced%20Materials%20-%202023%20-%20Jugovac.pdf
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