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001017310 0247_ $$2doi$$a10.1039/D3EE02540C
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001017310 0247_ $$2ISSN$$a1754-5706
001017310 0247_ $$2datacite_doi$$a10.34734/FZJ-2023-04044
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001017310 037__ $$aFZJ-2023-04044
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001017310 1001_ $$aZhang, Difei$$b0
001017310 245__ $$aObservation of reversible light degradation in organic photovoltaics induced by long-persistent radicals
001017310 260__ $$aCambridge$$bRSC Publ.$$c2023
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001017310 520__ $$aWith the rapid development of organic photovoltaics, device stability has become a crucial obstacle hindering their transition from laboratory-scale to industrial applications. However, it still remains unclear how light differs from heat in driving trap formation and device degradation. On the basis of the PTzBI-dF:Y6-BO system, it is observed that the post-thermal annealing on these high-performance organic solar cells can partially recover the light-induced burn-in losses. The recovery process is found to be correlated with a reversible charge extraction ability, reversible trap density of state, local charge carrier density and charge accumulation. Herein, we propose an innovative mechanism for light degradation in organic photovoltaic devices, which is triggered by the presence of light-induced long-persistent radicals. The findings offer deep insights into light degradation of organic photovoltaics and a new perspective for improving device stability under long-term operation.
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001017310 7001_ $$aLiu, Chao$$b1
001017310 7001_ $$aZhang, Kaicheng$$b2
001017310 7001_ $$aJia, Yanhua$$b3
001017310 7001_ $$00000-0001-8333-4898$$aZhong, Wenkai$$b4
001017310 7001_ $$aQiu, Weidong$$b5
001017310 7001_ $$00009-0002-9036-1469$$aLi, Yuanfeng$$b6
001017310 7001_ $$0P:(DE-Juel1)180635$$aHeumüller, Thomas$$b7$$ufzj
001017310 7001_ $$0P:(DE-Juel1)178784$$aForberich, Karen$$b8$$ufzj
001017310 7001_ $$aLe Corre, Vincent M.$$b9
001017310 7001_ $$aLüer, Larry$$b10
001017310 7001_ $$0P:(DE-Juel1)180778$$aLi, Ning$$b11$$eCorresponding author
001017310 7001_ $$00000-0001-9665-6642$$aHuang, Fei$$b12$$eCorresponding author
001017310 7001_ $$0P:(DE-Juel1)176427$$aBrabec, Christoph$$b13$$ufzj
001017310 7001_ $$00000-0003-1137-2355$$aYing, Lei$$b14$$eCorresponding author
001017310 773__ $$0PERI:(DE-600)2439879-2$$a10.1039/D3EE02540C$$gp. 10.1039.D3EE02540C$$n11$$p5339-5349 $$tEnergy & environmental science$$v16$$x1754-5692$$y2023
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