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@ARTICLE{Schlautmann:1017338,
      author       = {Schlautmann, Eva and Weiß, Alexander and Maus, Oliver and
                      Ketter, Lukas and Rana, Moumita and Puls, Sebastian and
                      Nickel, Vera and Gabbey, Christine and Hartnig, Christoph
                      and Bielefeld, Anja and Zeier, Wolfgang G.},
      title        = {{I}mpact of the {S}olid {E}lectrolyte {P}article {S}ize
                      {D}istribution in {S}ulfide‐{B}ased {S}olid‐{S}tate
                      {B}attery {C}omposites},
      journal      = {Advanced energy materials},
      volume       = {13},
      number       = {41},
      issn         = {1614-6832},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2023-04050},
      pages        = {2302309},
      year         = {2023},
      abstract     = {All solid-state batteries are promising, as they are
                      expected to offer increased energy density over conventional
                      lithium-ion batteries. Here, the microstructure of solid
                      composite electrodes plays a crucial role in determining the
                      characteristics of ionic and electronic pathways.
                      Microstructural aspects that impede charge carrier transport
                      can, for instance, be voids resulting from a general
                      mismatch of particle sizes. Solid electrolyte materials with
                      smaller particle size distribution represent a promising
                      approach to limit the formation of voids and to match the
                      smaller active materials. Therefore, a systematic
                      investigation on the influence of the solid electrolyte
                      particle size on the microstructural properties, charge
                      carrier transport, and rate performance is essential. This
                      study provides an understanding of the influence of the
                      particle sizes of Li6PS5Cl on the charge carrier transport
                      properties and their effect on the performance of
                      solid-state batteries. In conclusion, smaller Li6PS5Cl
                      particles optimize the charge transport properties and offer
                      a higher interface area with the active material, resulting
                      in improved solid-state battery performance.},
      cin          = {IEK-12},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001070485800001},
      doi          = {10.1002/aenm.202302309},
      url          = {https://juser.fz-juelich.de/record/1017338},
}