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@INBOOK{Mller:1017532,
author = {Müller, David},
title = {{NAP}-{XPS} {S}tudies of {M}ixed {C}onducting {E}lectrodes
{D}uring {H}igh-{T}emperature {E}lectrochemical {R}eactions},
volume = {21},
address = {London},
publisher = {WORLD SCIENTIFIC (EUROPE)},
reportid = {FZJ-2023-04181},
isbn = {978-1-80061-328-7 (print)},
series = {Catalytic Science Series},
pages = {457-499},
year = {2023},
comment = {Applications of X-ray Photoelectron Spectroscopy to
Catalytic Studies / Zafeiratos, Spyridon {CNRSFrance |
University of StrasbourgFrance} ; : WORLD SCIENTIFIC
(EUROPE), 2023, ; ISSN: 1793-1398=2399-4495 ; ISBN:
978-1-80061-328-7=978-1-80061-329-4 ; doi:10.1142/q0392},
booktitle = {Applications of X-ray Photoelectron
Spectroscopy to Catalytic Studies /
Zafeiratos, Spyridon {CNRSFrance |
University of StrasbourgFrance} ; :
WORLD SCIENTIFIC (EUROPE), 2023, ;
ISSN: 1793-1398=2399-4495 ; ISBN:
978-1-80061-328-7=978-1-80061-329-4 ;
doi:10.1142/q0392},
abstract = {In this chapter, we will give an overview of how NAP-XPS
can be used to investigate processes in and properties of
mixed ionic electronic conducting materials at elevated
temperatures, with a special focus on operando studies on
working electrochemical devices. After a brief introduction
of fundamental concepts of solid-state electroand defect
chemistry, we will focus on the reactions of prototypical
materials exposed to thermal, chemical, and electric stimuli
and how those can be elucidated with NAP-XPS. After
discussing the experimental challenges and general setups
used, we use examples to showcase the capabilities of
NAP-XPS. Starting with simple oxides, such as CeO2, where
NAP-XPS is used to clarify mechanisms of electrocatalytic
reactions with H2O and O2, we give several examples of how
the technique was used to significantly improve the
understanding of mixed conductors, the results themselves
being used to further drive technique development. NAP-XPS
shines brightly here, as surface-sensitive assessment of
both electrostatic as well as chemical properties is
unrivaled by any other technique. We extend the discussion
to more complex multicomponent transition metal perovskites
used in both cathodes and anodes of high-temperature
electrochemical devices, here the element and chemical state
sensitivity of NAP-XPS allows us to track atomic
rearrangements on the surface induced by changes in
electrochemical potentials, finishing with a short
description of NAP-XPS experiments on cermets, a special
case of a mixed conductor. This chapter is both intended for
the solid-state (electro)chemist to showcase how NAP-XPS
might help them to tackle physicochemical questions, as well
as to introduce the basic concepts of solid-state ionics and
electrochemistry to the spectroscopist, aiming to further
the understanding between those two fields.},
cin = {PGI-6},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / DFG project 319443528 -
Magnetfeldunterstützte chemische Gasphasenabscheidung von
Übergansmetalloxiden und in situ Untersuchungen der
elektronischen Struktur mit Hilfe von
Roentgenabsorptionsspektroskopie (MagSpec) (319443528)},
pid = {G:(DE-HGF)POF4-632 / G:(GEPRIS)319443528},
typ = {PUB:(DE-HGF)7},
url = {https://juser.fz-juelich.de/record/1017532},
}