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@ARTICLE{Rezaeyan:1018009,
      author       = {Rezaeyan, Amirsaman and Kampman, Niko and Pipich, Vitaliy
                      and Barnsley, Lester C. and Rother, Gernot and Magill,
                      Clayton and Ma, Jingsheng and Busch, Andreas},
      title        = {{E}volution of {P}ore {S}tructure in {O}rganic-{L}ean and
                      {O}rganic-{R}ich {M}udrocks},
      journal      = {Energy $\&$ fuels},
      volume       = {37},
      number       = {21},
      issn         = {0887-0624},
      address      = {Columbus, Ohio},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2023-04479},
      pages        = {16446 - 16460},
      year         = {2023},
      abstract     = {The pore structure of mudrocks is a key characteristic to
                      evaluate flow behavior through these rocks. Although
                      significant advances have been made to resolve pore
                      characteristics, porosity evolution, or pore connectivity,
                      there is still insufficient knowledge linking porosity
                      evolution to flow and transport in mudrocks. To better
                      understand these links, we conducted very small-angle
                      (VSANS) and small-angle neutron scattering (SANS)
                      experiments on 13 sets of mudrocks from global locations,
                      characterized by differences in composition, maturity, and
                      depositional environment. Our results indicate that a
                      homogeneous pore structure reflects a stable and low-energy
                      depositional environment. Organic-lean mudrocks mainly
                      contain pores <10 nm, which restricts flow and is beneficial
                      for, e.g., caprock seal integrity. Increasing maturity as a
                      result of increasing burial depth, and therefore,
                      temperature leads to porosity evolution. In organic-rich
                      mudrocks (ORMs), this happens through the generation of
                      organic matter pores and pore preservation around
                      diagenetically formed carbonates. ORMs mainly contain
                      macropores (>50 nm), favoring production from, e.g.,
                      unconventional reservoirs. SANS-derived pore size
                      distributions will help to better understand fluid
                      imbibition and flow properties in mudrocks through
                      comprehensive quantitative characterization of the nano- to
                      micron scale pore network conduits and their relationships
                      to burial diagenesis.},
      cin          = {JCNS-4 / JCNS-1 / MLZ / JCNS-FRM-II},
      ddc          = {660},
      cid          = {I:(DE-Juel1)JCNS-4-20201012 / I:(DE-Juel1)JCNS-1-20110106 /
                      I:(DE-588b)4597118-3 / I:(DE-Juel1)JCNS-FRM-II-20110218},
      pnm          = {632 - Materials – Quantum, Complex and Functional
                      Materials (POF4-632) / 6G4 - Jülich Centre for Neutron
                      Research (JCNS) (FZJ) (POF4-6G4)},
      pid          = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G4},
      experiment   = {EXP:(DE-MLZ)KWS3-20140101 / EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001098130200001},
      doi          = {10.1021/acs.energyfuels.3c02180},
      url          = {https://juser.fz-juelich.de/record/1018009},
}