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@ARTICLE{Dutta:1018017,
author = {Dutta, Rajesh and Thoma, Henrik and Sazonov, Andrew and
Náfrádi, Bálint and Meven, Martin and Gukasov, Arsen and
Kocsis, Vilmos and Zeitler, Uli and Puri, Alessandro and
Tokunaga, Yusuke and Taguchi, Yasujiro and Tokura, Yoshinori
and Bordács, Sándor and Kézsmárki, István and Hutanu,
Vladimir},
title = {{M}agnetic structure of the two-dimensional {XY}
antiferromagnet {S}r$_2${C}o{S}i$_2${O}$_7$ studied using
single-crystal neutron diffraction},
journal = {Physical review / B},
volume = {107},
number = {1},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2023-04487},
pages = {014420},
year = {2023},
abstract = {We report a combined polarized and unpolarized neutron
diffraction study on a multiferroic Sr$_2$CoSi$_2$O$_7$
(SCSO) single crystal below and above the antiferromagnetic
ordering temperature $T_N$ = 6.5 K. Unpolarized neutron
diffraction measurements at 15 K confirm the melilite-type
tetragonal $P\overline{4}2_1m$ space group as the parent
structure of SCSO. The low temperature study at 2.3 K, in
contrast, reveals symmetry lowering with the orthorhombic
Cmm′2′ and $P2_12′_12′$ magnetic space groups being
equally possible. In these $Cmm′2′$ and $P2_12′_12′$
magnetic space groups we obtain a very similar ordered
magnetic moment about 2.86 and 2.94μB/Co$^{2+}$,
respectively, which lies in the $ab$ plane. Our spin
polarized flipping ratio measurements under an applied
magnetic field of 6 T in the paramagnetic state support the
results of our bulk magnetization data, indicating strong
easy-plane spin anisotropy, responsible for the in-plane
order below $T_N$.},
cin = {JCNS-FRM-II / JARA-FIT / JCNS-2 / MLZ / JCNS-4},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-2-20110106 /
I:(DE-588b)4597118-3 / I:(DE-Juel1)JCNS-4-20201012},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000927608900003},
doi = {10.1103/PhysRevB.107.014420},
url = {https://juser.fz-juelich.de/record/1018017},
}