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@ARTICLE{Bosoni:1018070,
author = {Bosoni, Emanuele and Beal, Louis and Bercx, Marnik and
Blaha, Peter and Blügel, Stefan and Bröder, Jens and
Callsen, Martin and Cottenier, Stefaan and Degomme, Augustin
and Dikan, Vladimir and Eimre, Kristjan and Flage-Larsen,
Espen and Fornari, Marco and Garcia, Alberto and Genovese,
Luigi and Giantomassi, Matteo and Huber, Sebastiaan P. and
Janssen, Henning and Kastlunger, Georg and Krack, Matthias
and Kresse, Georg and Kühne, Thomas D. and Lejaeghere, Kurt
and Madsen, Georg K. H. and Marsman, Martijn and Marzari,
Nicola and Michalicek, Gregor and Mirhosseini, Hossein and
Müller, Tiziano M. A. and Petretto, Guido and Pickard,
Chris J. and Poncé, Samuel and Rignanese, Gian-Marco and
Rubel, Oleg and Ruh, Thomas and Sluydts, Michael and
Vanpoucke, Danny E. P. and Vijay, Sudarshan and Wolloch,
Michael and Wortmann, Daniel and Yakutovich, Aliaksandr V.
and Yu, Jusong and Zadoks, Austin and Zhu, Bonan and Pizzi,
Giovanni},
title = {{H}ow to verify the precision of density-functional-theory
implementations via reproducible and universal workflows},
journal = {Nature reviews / Physics},
volume = {6},
issn = {2522-5820},
address = {London},
publisher = {Springer Nature},
reportid = {FZJ-2023-04521},
pages = {45-58},
year = {2024},
abstract = {Density-functional theory methods and codes adopting
periodic boundary conditions are extensively used in
condensed matter physics and materials science research. In
2016, their precision (how well properties computed with
different codes agree among each other) was systematically
assessed on elemental crystals: a first crucial step to
evaluate the reliability of such computations. In this
Expert Recommendation, we discuss recommendations for
verification studies aiming at further testing precision and
transferability of density-functional-theory computational
approaches and codes. We illustrate such recommendations
using a greatly expanded protocol covering the whole
periodic table from Z = 1 to 96 and characterizing 10
prototypical cubic compounds for each element: four unaries
and six oxides, spanning a wide range of coordination
numbers and oxidation states. The primary outcome is a
reference dataset of 960 equations of state cross-checked
between two all-electron codes, then used to verify and
improve nine pseudopotential-based approaches. Finally, we
discuss the extent to which the current results for total
energies can be reused for different goals.},
cin = {PGI-1 / IAS-1 / JARA-FIT / JARA-HPC / IAS-9},
ddc = {530},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$ /
I:(DE-Juel1)IAS-9-20201008},
pnm = {5211 - Topological Matter (POF4-521) / 5111 -
Domain-Specific Simulation $\&$ Data Life Cycle Labs (SDLs)
and Research Groups (POF4-511) / MaX - MAterials design at
the eXascale. European Centre of Excellence in materials
modelling, simulations, and design (824143) / Helmholtz
Platform for Research Software Engineering - Preparatory
Study $(HiRSE_PS-20220812)$ / AIDAS - Joint Virtual
Laboratory for AI, Data Analytics and Scalable Simulation
$(aidas_20200731)$},
pid = {G:(DE-HGF)POF4-5211 / G:(DE-HGF)POF4-5111 /
G:(EU-Grant)824143 / $G:(DE-Juel-1)HiRSE_PS-20220812$ /
$G:(DE-Juel-1)aidas_20200731$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001103174800001},
doi = {10.1038/s42254-023-00655-3},
url = {https://juser.fz-juelich.de/record/1018070},
}