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@INPROCEEDINGS{Zeng:1018118,
author = {Zeng, Yuan and Schäfer, Laura-Alena and Guillon, Olivier
and Ivanova, Mariya and Menzler, Norbert H.},
title = {{T}ailoring {P}roperties of {B}a{Z}r0.8-x{C}e0.2{Y}x{O}3-δ
{P}roton {C}onductors for {E}nhanced {P}erformance in
{E}lectrochemical {D}evices},
reportid = {FZJ-2023-04562},
year = {2023},
abstract = {Solid oxide fuel and electrolysis cells (SOFC/SOEC) based
on ceramic proton conductors efficiently convert chemical
energy into electricity and vice versa at intermediate
operating temperatures (400-600 °C)[1]. Acceptor doped
BaCeO3 and BaZrO3, are the most extensively studied proton
conductors. BaCeO3 exhibits high proton conductivity but
shows lower chemical stability in H2O and CO2 environments.
Conversely, BaZrO3 possesses higher chemical stability but
lower proton transport ability at the grain boundaries[2].
Preparing Ba(Zr,Ce)O3 solid solutions with the appropriate
Zr/Ce ratio at the B-site in the perovskite crystal
structure is a compromise strategy. In this work, 20
$mol.\%$ of Ce was introduced into the lattice of Y-doped
BaZrO3, and 0.5 $wt.\%$ of NiO was applied as a sintering
aid. The Y2O3 substituent amount varies within the range of
10-30 $mol.\%$ in order to study the influence of Y on the
phase formation, microstructure, hydration behavior and
electrical performance. Y-riched phase has been found in
samples with Y content exceeding 25 $mol.\%.$ And excessive
Y2O3 substitution has a negative impact on the grain
boundary conductivity. In addition, mechanical performance
and thermo-chemical stability is also taken into
consideration to evaluate the suitability of this material
for electrochemical devices.},
month = {Sep},
date = {2023-09-16},
organization = {The 21st International Conference on
Solid-State Protonic Conductors,
Fukuoka (Japan), 16 Sep 2023 - 22 Sep
2023},
subtyp = {After Call},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / SOFC -
Solid Oxide Fuel Cell (SOFC-20140602)},
pid = {G:(DE-HGF)POF4-1231 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)24},
url = {https://juser.fz-juelich.de/record/1018118},
}