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001018241 1001_ $$0P:(DE-HGF)0$$aNoei, Neda$$b0
001018241 245__ $$aManipulating the Spin Orientation of Co Atoms Using Monatomic Cu Chains
001018241 260__ $$aWashington, DC$$bACS Publ.$$c2023
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001018241 520__ $$aHarnessing the spin of single atoms is at the heart of quantum information nanotechnology based on magnetic concepts. By attaching single Co atoms to monatomic Cu chains, we demonstrate the ability to control the spin orientation by the atomic environment. Due to spin–orbit coupling (SOC), the spin is tilted by ≈58° from the surface normal toward the chain as evidenced by inelastic tunneling spectroscopy. These findings are reproduced by density functional theory calculations and have implications for Co atoms on pristine Cu(111), which are believed to be Kondo systems. Our quantum Monte Carlo calculations suggest that SOC suppresses the Kondo effect of Co atoms at chains and on the flat surface. Our work impacts the fundamental understanding of low-energy excitations in nanostructures on surfaces and demonstrates the ability to manipulate atomic-scale magnetic moments, which can have tremendous implications for quantum devices.
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001018241 536__ $$0G:(EU-Grant)681405$$aDynasore - Dynamical magnetic excitations with spin-orbit interaction in realistic nanostructures (681405)$$c681405$$fERC-2015-CoG$$x2
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001018241 7001_ $$0P:(DE-HGF)0$$aMozara, Roberto$$b1
001018241 7001_ $$0P:(DE-Juel1)178851$$aMontero, Ana$$b2
001018241 7001_ $$0P:(DE-Juel1)168211$$aBrinker, Sascha$$b3
001018241 7001_ $$0P:(DE-HGF)0$$aIde, Niklas$$b4
001018241 7001_ $$0P:(DE-Juel1)162225$$aGuimaraes, Filipe$$b5$$ufzj
001018241 7001_ $$0P:(DE-HGF)0$$aLichtenstein, Alexander I.$$b6
001018241 7001_ $$0P:(DE-HGF)0$$aBerndt, Richard$$b7
001018241 7001_ $$0P:(DE-Juel1)130805$$aLounis, Samir$$b8$$ufzj
001018241 7001_ $$0P:(DE-HGF)0$$aWeismann, Alexander$$b9$$eCorresponding author
001018241 773__ $$0PERI:(DE-600)2048866-X$$a10.1021/acs.nanolett.3c02532$$gVol. 23, no. 19, p. 8988 - 8994$$n19$$p8988 - 8994$$tNano letters$$v23$$x1530-6984$$y2023
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001018241 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$a Institut für Experimentelle und Angewandte Physik, Christian-Albrechts-Universität zu Kiel, 24098 Kiel, Germany$$b0
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001018241 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$a Institut für Experimentelle und Angewandte Physik, Christian-Albrechts-Universität zu Kiel, 24098 Kiel, Germany$$b4
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