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@ARTICLE{Noei:1018241,
author = {Noei, Neda and Mozara, Roberto and Montero, Ana and
Brinker, Sascha and Ide, Niklas and Guimaraes, Filipe and
Lichtenstein, Alexander I. and Berndt, Richard and Lounis,
Samir and Weismann, Alexander},
title = {{M}anipulating the {S}pin {O}rientation of {C}o {A}toms
{U}sing {M}onatomic {C}u {C}hains},
journal = {Nano letters},
volume = {23},
number = {19},
issn = {1530-6984},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {FZJ-2023-04637},
pages = {8988 - 8994},
year = {2023},
note = {Bitte Post-print ergänzen},
abstract = {Harnessing the spin of single atoms is at the heart of
quantum information nanotechnology based on magnetic
concepts. By attaching single Co atoms to monatomic Cu
chains, we demonstrate the ability to control the spin
orientation by the atomic environment. Due to spin–orbit
coupling (SOC), the spin is tilted by ≈58° from the
surface normal toward the chain as evidenced by inelastic
tunneling spectroscopy. These findings are reproduced by
density functional theory calculations and have implications
for Co atoms on pristine Cu(111), which are believed to be
Kondo systems. Our quantum Monte Carlo calculations suggest
that SOC suppresses the Kondo effect of Co atoms at chains
and on the flat surface. Our work impacts the fundamental
understanding of low-energy excitations in nanostructures on
surfaces and demonstrates the ability to manipulate
atomic-scale magnetic moments, which can have tremendous
implications for quantum devices.},
cin = {PGI-1 / IAS-1 / JSC},
ddc = {660},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406 /
I:(DE-Juel1)JSC-20090406},
pnm = {5211 - Topological Matter (POF4-521) / 5112 - Cross-Domain
Algorithms, Tools, Methods Labs (ATMLs) and Research Groups
(POF4-511) / Dynasore - Dynamical magnetic excitations with
spin-orbit interaction in realistic nanostructures (681405)},
pid = {G:(DE-HGF)POF4-5211 / G:(DE-HGF)POF4-5112 /
G:(EU-Grant)681405},
typ = {PUB:(DE-HGF)16},
pubmed = {37782684},
UT = {WOS:001076073900001},
doi = {10.1021/acs.nanolett.3c02532},
url = {https://juser.fz-juelich.de/record/1018241},
}