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@ARTICLE{Ebert:1018243,
author = {Ebert, Julian and Jennings, Dylan and Schäfer, Laura-Alena
and Sebold, Doris and Rheinheimer, Wolfgang},
title = {{B}ulk and grain boundary conductivity in doped
{B}a{Z}r{O}3: {B}ulk contribution dominates at operating
temperatures},
journal = {Scripta materialia},
volume = {241},
issn = {1359-6462},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2023-04639},
pages = {115852 -},
year = {2024},
note = {Paper ist Gold Open AccessWeitere Grants sind:Emmy Noether
Programme under contract no. Rh 146/1–1Helmholtz
Association of German Research Centers (HGF) and the Federal
Ministry of Education and Research (BMBF), Innovation Pool
project “Solar H2: Highly Pure and Compressed”},
abstract = {This study evaluates the role of microstructure for the
conductivity of BaZrO3-based protonic conductors. Bulk
conductivity was found to be the limiting conductivity
contribution in BaZr0.8Y0.2O3-δ (BZY20) and
BaZr0.7Ce0.2Y0.1O3-δ (BZCY72) at operating temperatures.
The effective grain boundary conductivity only dominates the
total conductivity below a crossover point (200 °C for
BZY20, 150 °C for BZCY72). The crossover point was
determined by using a well-calibrated electrochemical
impedance spectroscopy setup to measure from 600 °C to 50
°C with up to 10 MHz. As such, bulk and grain boundary
could be fitted separately up to 350 °C instead of 200 °C,
as often seen in literature. According to these results, the
impact of grain boundaries on the total conductivity of
BZY20 and BZCY72 at operating temperature might be less than
assumed. Therefore, research should not only focus on
increasing the conductivity of the grain boundary, but also
on maximizing the bulk conductivity.},
cin = {IEK-1},
ddc = {670},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / SFB 1548
B04 - Einfluss der grundlegenden elektronischen Struktur auf
die Korngrenzeigenschaften in oxidischen Perowskiten (B04)
(513417808)},
pid = {G:(DE-HGF)POF4-1231 / G:(GEPRIS)513417808},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001161533200001},
doi = {10.1016/j.scriptamat.2023.115852},
url = {https://juser.fz-juelich.de/record/1018243},
}