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@ARTICLE{GaraiMarin:1018441,
      author       = {Garai-Marin, Haritz and Dias, Manuel dos Santos and Lounis,
                      Samir and Ibañez-Azpiroz, Julen and Eiguren, Asier},
      title        = {{M}icroscopic theory of spin relaxation of a single {F}e
                      adatom coupled to substrate vibrations},
      journal      = {Physical review / B},
      volume       = {107},
      number       = {14},
      issn         = {2469-9950},
      address      = {Woodbury, NY},
      publisher    = {Inst.},
      reportid     = {FZJ-2023-04816},
      pages        = {144417},
      year         = {2023},
      abstract     = {Understanding the spin-relaxation mechanism of single
                      adatoms is an essential step towards creating atomic
                      magnetic memory bits or even qubits. Here, we present an
                      essentially parameter-free theory by combining ab initio
                      electronic and vibrational properties with the many-body
                      nature of atomic states. Our calculations account for the
                      millisecond spin lifetime measured recently on Fe adatoms on
                      MgO/Ag(100) and reproduce the dependence on the number of
                      decoupling layers and the external magnetic field. We show
                      how the atomic interaction with the environment should be
                      tuned in order to enhance the magnetic stability, and
                      propose a clear fingerprint for experimentally detecting a
                      localized spin-phonon excitation.},
      cin          = {PGI-1 / IAS-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406},
      pnm          = {5211 - Topological Matter (POF4-521)},
      pid          = {G:(DE-HGF)POF4-5211},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000976430400005},
      doi          = {10.1103/PhysRevB.107.144417},
      url          = {https://juser.fz-juelich.de/record/1018441},
}