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001     1018441
005     20231213115703.0
024 7 _ |a 10.1103/PhysRevB.107.144417
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024 7 _ |a 10.34734/FZJ-2023-04816
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100 1 _ |a Garai-Marin, Haritz
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245 _ _ |a Microscopic theory of spin relaxation of a single Fe adatom coupled to substrate vibrations
260 _ _ |a Woodbury, NY
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520 _ _ |a Understanding the spin-relaxation mechanism of single adatoms is an essential step towards creating atomic magnetic memory bits or even qubits. Here, we present an essentially parameter-free theory by combining ab initio electronic and vibrational properties with the many-body nature of atomic states. Our calculations account for the millisecond spin lifetime measured recently on Fe adatoms on MgO/Ag(100) and reproduce the dependence on the number of decoupling layers and the external magnetic field. We show how the atomic interaction with the environment should be tuned in order to enhance the magnetic stability, and propose a clear fingerprint for experimentally detecting a localized spin-phonon excitation.
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700 1 _ |a Dias, Manuel dos Santos
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700 1 _ |a Lounis, Samir
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700 1 _ |a Ibañez-Azpiroz, Julen
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700 1 _ |a Eiguren, Asier
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773 _ _ |a 10.1103/PhysRevB.107.144417
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856 4 _ |u https://juser.fz-juelich.de/record/1018441/files/PhysRevB.107.144417.pdf
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910 1 _ |a Physics Department, University of the Basque Country UPV/EHU, 48080 Bilbao, Basque Country, Spain
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910 1 _ |a Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián, Spain
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910 1 _ |a Forschungszentrum Jülich
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910 1 _ |a Faculty of Physics, University of Duisburg-Essen & CENIDE, 47053 Duisburg, Germany
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910 1 _ |a Scientific Computing Department, STFC Daresbury Laboratory, Warrington WA4 4AD, United Kingdom
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910 1 _ |a Centro de Física de Materiales, Universidad del País Vasco UPV/EHU, 20018 San Sebastián, Spain
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910 1 _ |a EHU Quantum Center, University of the Basque Country UPV/EHU, 48940 Leioa, Spain
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