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| 001 | 1018986 | ||
| 005 | 20250204113740.0 | ||
| 024 | 7 | _ | |a 10.1002/cssc.202301398 |2 doi |
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| 100 | 1 | _ | |a Veenstra, Florentine LP |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a CO2 electroreduction to syngas with tunable composition in an artificial leaf |
| 260 | _ | _ | |a Weinheim |c 2024 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 500 | _ | _ | |a Bitte Post-print ergänzen |
| 520 | _ | _ | |a Artificial leaves (a-leaves) can reduce carbon dioxide into syngas using solar power and could be combined with thermo- and biocatalytic technologies to decentralize the production of valuable products. By providing variable CO:H2 ratios on demand, a-leaves could facilitate optimal combinations and control the distribution of products in most of these hybrid systems. However, the current design procedures of a-leaves concentrate on achieving high performance for a predetermined syngas composition. This study demonstrates that incorporating the electrolyte flow as a design variable enables flexible production without compromising performance. The concept was tested on an a-leaf using a commercial cell, a Cu2O:Inx cathodic catalyst, and an inexpensive amorphous silicon thin-film photovoltaic module. Syngas with CO:H2ratio in the range of 1.8-2.3 could be attained with only 2% deviation from the optimal cell voltage and controllable solely by catholyte flow. These features could be beneficial for downstream technologies such as Fischer Tropsch synthesis and anaerobic fermentation. |
| 536 | _ | _ | |a 1213 - Cell Design and Development (POF4-121) |0 G:(DE-HGF)POF4-1213 |c POF4-121 |f POF IV |x 0 |
| 536 | _ | _ | |a A-LEAF - An Artificial Leaf: a photo-electro-catalytic cell from earth-abundant materials for sustainable solar production of CO2-based chemicals and fuels (732840) |0 G:(EU-Grant)732840 |c 732840 |f FETPROACT-2016 |x 1 |
| 588 | _ | _ | |a Dataset connected to CrossRef, Journals: juser.fz-juelich.de |
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| 700 | 1 | _ | |a Martín, Antonio J |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Weigand, Daniel |0 P:(DE-Juel1)130302 |b 3 |u fzj |
| 700 | 1 | _ | |a Kirchhoff, Joachim |0 P:(DE-Juel1)130256 |b 4 |u fzj |
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| 700 | 1 | _ | |a Pérez-Ramírez, Javier |0 P:(DE-HGF)0 |b 7 |
| 773 | _ | _ | |a 10.1002/cssc.202301398 |g p. e202301398 |0 PERI:(DE-600)2411405-4 |p e202301398 |t ChemSusChem |v 1864-5631 |y 2024 |x 1864-5631 |
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