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@ARTICLE{Ortmann:1019450,
author = {Ortmann, Till and Fuchs, Till and Eckhardt, Janis K. and
Ding, Ziming and Ma, Qianli and Tietz, Frank and Kübel,
Christian and Rohnke, Marcus and Janek, Jürgen},
title = {{D}eposition of {S}odium {M}etal at the
{C}opper‐{N}a{SICON} {I}nterface for {R}eservoir‐{F}ree
{S}olid‐{S}tate {S}odium {B}atteries},
journal = {Advanced energy materials},
volume = {14},
number = {5},
issn = {1614-6832},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2023-05400},
pages = {2302729},
year = {2024},
abstract = {“Anode-free” solid-state battery concepts are explored
extensively as theypromise a higher energy density with less
material consumption and simpleanode processing. Here, the
homogeneous and uniform electrochemicaldeposition of alkali
metal at the interface between current collector and
solidelectrolyte plays the central role to form a metal
anode within the first cycle.While the cathodic deposition
of lithium has been studied intensively,knowledge on sodium
deposition is scarce. In this work, dense and uniformsodium
layers of several microns thickness are deposited at
theCu|Na3.4Zr2Si2.4P0.6O12 interface with high
reproducibility. At current densitiesof ≈1 mA∙cm−2,
relatively uniform coverage is achieved underneath
thecurrent collector, as shown by electrochemical impedance
spectroscopy and3D confocal microscopy. In contrast, only
slight variations of the coverage areobserved at different
stack pressures. Early stages of the sodium metal growthare
analyzed by in situ transmission electron microscopy
revealing orientedgrowth of sodium. The results demonstrate
that reservoir-free (“anode-free”)sodium-based batteries
are feasible and may stimulate further research effortsin
sodium-based solid-state batteries.},
cin = {IEK-1},
ddc = {050},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1222 - Components and Cells (POF4-122) / 1221 -
Fundamentals and Materials (POF4-122)},
pid = {G:(DE-HGF)POF4-1222 / G:(DE-HGF)POF4-1221},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001115802400001},
doi = {10.1002/aenm.202302729},
url = {https://juser.fz-juelich.de/record/1019450},
}