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@ARTICLE{Khn:1019492,
      author       = {Kühn, Sebastian P. and Weiling, Matthias and Diddens,
                      Diddo and Baghernejad, Masoud and Winter, Martin and
                      Cekic-Laskovic, Isidora},
      title        = {{I}mpact of in coin cell atmosphere on lithium metal
                      battery performance},
      journal      = {Energy Materials},
      volume       = {3},
      issn         = {2770-5900},
      address      = {Alhambra CA},
      publisher    = {[Verlag nicht ermittelbar]},
      reportid     = {FZJ-2023-05439},
      pages        = {3000020},
      year         = {2023},
      abstract     = {Research on lithium metal as a high-capacity anode for
                      future lithium metal batteries (LMBs) is currently at an
                      all-time high. To date, the different influences of a highly
                      pure argon glovebox (GB) and an industry-relevant ambient
                      dry room (DR) atmosphere have received little attention in
                      the scientific community. In this paper, we report on the
                      impact of in coin cell atmosphere (ICCA) on the performance
                      of an LMB as well as its interphase characteristics and
                      properties in combination with three organic carbonate-based
                      electrolytes with and without two well-known
                      interphase-forming additives, namely fluoroethylene
                      carbonate (FEC) and vinylene carbonate (VC). The results
                      obtained from this carefully executed systematic study show
                      a substantial impact of the ICCA on solid electrolyte
                      interphase (SEI) resistance (RSEI) and lithium
                      stripping/plating homogeneity. In a transition metal cathode
                      (NMC811) containing LMBs, a DR ICCA results in an up to
                      $50\%$ increase in lifetime due to the improved chemical
                      composition of the cathode electrolyte interphase (CEI).
                      Furthermore, different impacts on electrode characteristics
                      and cell performance were observed depending on the utilized
                      functional additive. Since this study focuses on a largely
                      overlooked influential factor of LMB performance, it
                      highlights the importance of comparability and transparency
                      in published research and the importance of taking
                      differences between research and industrial environments
                      into consideration in the aim of establishing and
                      commercializing LMB cell components.},
      cin          = {IEK-12},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1222 - Components and Cells (POF4-122) / Lillint -
                      Thermodynamic and kinetic stability of the Lithium-Liquid
                      Electrolyte Interface (13XP0225B)},
      pid          = {G:(DE-HGF)POF4-1222 / G:(BMBF)13XP0225B},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001108912800004},
      doi          = {10.20517/energymater.2023.07},
      url          = {https://juser.fz-juelich.de/record/1019492},
}