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@ARTICLE{Jiang:1019517,
      author       = {Jiang, Lihua and Cheng, Yuan and Wang, Shuping and Cheng,
                      Yifeng and Jin, Kaiqiang and Sun, Jinhua and Winter, Martin
                      and Cekic-Laskovic, Isidora and Wang, Qingsong},
      title        = {{A} nonflammable diethyl ethylphosphonate-based electrolyte
                      improved by synergistic effect of lithium
                      difluoro(oxalato)borate and fluoroethylene carbonate},
      journal      = {Journal of power sources},
      volume       = {570},
      issn         = {0378-7753},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2023-05464},
      pages        = {233051 -},
      year         = {2023},
      abstract     = {The vital physical and chemical properties of the lithium
                      conducting salt, solvent/co-solvent and functionaladditive
                      determine the overall properties and performance of the
                      resulting electrolyte formulation. Explorationson right
                      combinations of the carefully selected electrolyte
                      components are expected to further balance
                      theelectrochemical and safety performances of chosen
                      electrolyte formulations in given cell chemistries. In
                      thisstudy, a new nonaqueous aprotic electrolyte is designed
                      by using lithium difluoro(oxalato)borate (LiODFB)
                      asconducting salt, diethyl ethylphosphonate (DEEP) as
                      solvent, and fluoroethylene carbonate (FEC) as co-solvent
                      toachieve a nonflammable electrolyte formulation with
                      competent electrochemical performance. The LiODFB andFEC are
                      believed to take part in complex interfacial interactions
                      with a synergistic effect. LiNi0.8Co0.1Mn0.1O2(NCM811)‖Li
                      cells using the optimized electrolyte formulation of 1.3 M
                      LiODFB/DEEP $30\%$ FEC exhibits a stablelong-term cycling
                      performance at 1.0 C with a reversible average specific
                      discharge capacity of 169.5 mAh g􀀀 1during 100 cycles,
                      which is comparable to cells using commercial electrolytes.
                      Furthermore, the 1.3 M LiODFB/DEEP $30\%$ FEC electrolyte
                      shows good thermal stability and effectively reduces the
                      heat generation duringthermal decomposition of NCM811
                      cathode. The results provide a good reference for the design
                      of next generationof safe, nonflammable electrolytes for
                      lithium-based battery application.},
      cin          = {IEK-12},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001054211000001},
      doi          = {10.1016/j.jpowsour.2023.233051},
      url          = {https://juser.fz-juelich.de/record/1019517},
}