TY  - JOUR
AU  - Duncan, Atkins
AU  - Elixabete, Ayerbe
AU  - Benayad, Anass
AU  - Capone, Federico G.
AU  - Enio, Capria
AU  - Ivano, Casteli E.
AU  - Cekic-Laskovic, Isidora
AU  - Raul, Ciria
AU  - Dudy, Lenart
AU  - Edström, Kristina
AU  - Johnson, Mark R.
AU  - Li, Hongjiao
AU  - Lastra, Juan Maria Garcia
AU  - Souza, Matheus Leal De
AU  - Meunier, Valentin
AU  - Morcrette, Mathieu
AU  - Reichert, Harald
AU  - Simon, Patrice
AU  - Rueff, Jean-Pascal
AU  - Sottmann, Jonas
AU  - Wenzel, Wolfgang
AU  - Grimaud, Alexis
TI  - Understanding Battery Interfaces by Combined Characterizationand Simulation Approaches: Challenges and Perspectives
JO  - Advanced energy materials
VL  - 12
IS  - 17
SN  - 1614-6832
CY  - Weinheim
PB  - Wiley-VCH
M1  - FZJ-2023-05469
SP  - 2102687
PY  - 2022
AB  - Driven by the continuous search for improving performances, understandingthe phenomena at the electrode/electrolyte interfaces has become an overridingfactor for the success of sustainable and efficient battery technologiesfor mobile and stationary applications. Toward this goal, rapid advances havebeen made regarding simulations/modeling techniques and characterizationapproaches, including high-throughput electrochemical measurementscoupled with spectroscopies. Focusing on Li-ion batteries, current developmentsare analyzed in the field as well as future challenges in order to gaina full description of interfacial processes across multiple length/timescales;from charge transfer to migration/diffusion properties and interphases formation,up to and including their stability over the entire battery lifetime. Forsuch complex and interrelated phenomena, developing a unified workflowintimately combining the ensemble of these techniques will be critical tounlocking their full investigative potential. For this paradigm shift in batterydesign to become reality, it necessitates the implementation of researchstandards and protocols, underlining the importance of a concerted approachacross the community. With this in mind, major collaborative initiatives gatheringcomplementary strengths and skills will be fundamental if societal andenvironmental imperatives in this domain are to be met.
LB  - PUB:(DE-HGF)16
UR  - <Go to ISI:>//WOS:000731410500001
DO  - DOI:10.1002/aenm.202102687
UR  - https://juser.fz-juelich.de/record/1019522
ER  -