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@ARTICLE{Duncan:1019522,
author = {Duncan, Atkins and Elixabete, Ayerbe and Benayad, Anass and
Capone, Federico G. and Enio, Capria and Ivano, Casteli E.
and Cekic-Laskovic, Isidora and Raul, Ciria and Dudy, Lenart
and Edström, Kristina and Johnson, Mark R. and Li, Hongjiao
and Lastra, Juan Maria Garcia and Souza, Matheus Leal De and
Meunier, Valentin and Morcrette, Mathieu and Reichert,
Harald and Simon, Patrice and Rueff, Jean-Pascal and
Sottmann, Jonas and Wenzel, Wolfgang and Grimaud, Alexis},
title = {{U}nderstanding {B}attery {I}nterfaces by {C}ombined
{C}haracterizationand {S}imulation {A}pproaches:
{C}hallenges and {P}erspectives},
journal = {Advanced energy materials},
volume = {12},
number = {17},
issn = {1614-6832},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2023-05469},
pages = {2102687},
year = {2022},
abstract = {Driven by the continuous search for improving performances,
understandingthe phenomena at the electrode/electrolyte
interfaces has become an overridingfactor for the success of
sustainable and efficient battery technologiesfor mobile and
stationary applications. Toward this goal, rapid advances
havebeen made regarding simulations/modeling techniques and
characterizationapproaches, including high-throughput
electrochemical measurementscoupled with spectroscopies.
Focusing on Li-ion batteries, current developmentsare
analyzed in the field as well as future challenges in order
to gaina full description of interfacial processes across
multiple length/timescales;from charge transfer to
migration/diffusion properties and interphases formation,up
to and including their stability over the entire battery
lifetime. Forsuch complex and interrelated phenomena,
developing a unified workflowintimately combining the
ensemble of these techniques will be critical tounlocking
their full investigative potential. For this paradigm shift
in batterydesign to become reality, it necessitates the
implementation of researchstandards and protocols,
underlining the importance of a concerted approachacross the
community. With this in mind, major collaborative
initiatives gatheringcomplementary strengths and skills will
be fundamental if societal andenvironmental imperatives in
this domain are to be met.},
cin = {IEK-12},
ddc = {050},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1222 - Components and Cells (POF4-122) / BIG-MAP - Battery
Interface Genome - Materials Acceleration Platform (957189)
/ BATTERY 2030PLUS - BATTERY 2030+ large-scale research
initiative: At the heart of a connected green society
(957213)},
pid = {G:(DE-HGF)POF4-1222 / G:(EU-Grant)957189 /
G:(EU-Grant)957213},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000731410500001},
doi = {10.1002/aenm.202102687},
url = {https://juser.fz-juelich.de/record/1019522},
}