001     1019896
005     20240709082038.0
037 _ _ |a FZJ-2023-05717
100 1 _ |a Mänken, Christian
|0 P:(DE-Juel1)188978
|b 0
|e Corresponding author
|u fzj
111 2 _ |a 18th International Symposium on Solid Oxide Fuel Cells
|g SOFC-XVIII
|c Boston
|d 2023-05-28 - 2023-06-02
|w USA
245 _ _ |a Solid Oxide Cell State-of-Health Prediction with Machine Learning
260 _ _ |c 2023
336 7 _ |a Conference Paper
|0 33
|2 EndNote
336 7 _ |a INPROCEEDINGS
|2 BibTeX
336 7 _ |a conferenceObject
|2 DRIVER
336 7 _ |a CONFERENCE_POSTER
|2 ORCID
336 7 _ |a Output Types/Conference Poster
|2 DataCite
336 7 _ |a Poster
|b poster
|m poster
|0 PUB:(DE-HGF)24
|s 1704184604_26653
|2 PUB:(DE-HGF)
|x After Call
520 _ _ |a To better understand degradation in electrochemical converters and helping to correlate certain phenomena with specific operating conditions, machine learning (ML) methods are increasingly being applied. Success has already been achieved in the field of degradation analysis and prediction of capacity of Lithium ion batteries [1], for instance. In terms of Solix Oxide Cell (SOC) stacks ML methods have been applied mainly with the aim of identification of faulty operation modes and degradation related fault diagnosis [2]. ML approaches usually require a considerable amount of real training data, when used for forecasting models. A data consolidation and curation strategy was developed with the aim of processing the historic long-term test bench data of SOCs collected by Forschungszentrum Jülich over the past years. In comparison to other datasets developed in this field [3], the one presented in this work contains SOC stack tests in fuel cell operation with significantly longer operating times under load. A compilation of the sample experiments and the consolidation into a hierarchical data format are presented. Further, an essential part of the strategy is the automatic curation and analysis of electrochemical impedance spectroscopy (EIS) measurements, using a specifically developed procedure in Python. The varying quality of measurements from past years, as well as recurring artefacts such as parasitic inductances, can be addressed in this way. Additional distribution of relaxation times (DRT) deconvolutions and equivalent circuit modelling (ECM) are performed, as part of the procedure to automatically retrieve feature values from measurements. The novel dataset, which to the authors’ knowledge includes some of the longest SOC stack tests available, serves as the basis for several evaluations. In addition to classification and clustering work to derive degradation patterns, in particular based on the EIS data, another focus is on the development of forecasting models. The current work is primarily concerned with long short-term memory (LSTM), as well as regression models that make use of both the time series data and the characterisation measurements, such as EIS. References:[1]: Jones, P.K., Stimming, U. & Lee, A.A. Impedance-based forecasting of lithium-ion battery performance amid uneven usage. Nat Commun 13, 4806 (2022). [2]: B. Yang et al. Solid oxide fuel cell systems fault diagnosis: Critical summarization, classification, and perspectives. Journal of Energy Storage 34, 102153 (2021)[3]: A.K. Padinjarethil, S. Pollok & A. Hagen. Degradation studies using machine learning on novel solid oxide cell database. Fuel Cells. 21, 566–576 (2021)
536 _ _ |a 1231 - Electrochemistry for Hydrogen (POF4-123)
|0 G:(DE-HGF)POF4-1231
|c POF4-123
|f POF IV
|x 0
536 _ _ |a HITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406)
|0 G:(DE-Juel1)HITEC-20170406
|c HITEC-20170406
|x 1
650 1 7 |a Energy
|0 V:(DE-MLZ)GC-110
|2 V:(DE-HGF)
|x 0
700 1 _ |a Schäfer, Christian
|0 P:(DE-Juel1)201475
|b 1
700 1 _ |a Kunz, Felix
|0 P:(DE-Juel1)192282
|b 2
700 1 _ |a Eichel, Rüdiger-A.
|0 P:(DE-Juel1)156123
|b 3
|e Thesis advisor
|u fzj
909 C O |o oai:juser.fz-juelich.de:1019896
|p VDB
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 0
|6 P:(DE-Juel1)188978
910 1 _ |a RWTH Aachen
|0 I:(DE-588b)36225-6
|k RWTH
|b 0
|6 P:(DE-Juel1)188978
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 1
|6 P:(DE-Juel1)201475
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 2
|6 P:(DE-Juel1)192282
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 3
|6 P:(DE-Juel1)156123
910 1 _ |a RWTH Aachen
|0 I:(DE-588b)36225-6
|k RWTH
|b 3
|6 P:(DE-Juel1)156123
913 1 _ |a DE-HGF
|b Forschungsbereich Energie
|l Materialien und Technologien für die Energiewende (MTET)
|1 G:(DE-HGF)POF4-120
|0 G:(DE-HGF)POF4-123
|3 G:(DE-HGF)POF4
|2 G:(DE-HGF)POF4-100
|4 G:(DE-HGF)POF
|v Chemische Energieträger
|9 G:(DE-HGF)POF4-1231
|x 0
914 1 _ |y 2023
920 _ _ |l yes
920 1 _ |0 I:(DE-Juel1)IEK-9-20110218
|k IEK-9
|l Grundlagen der Elektrochemie
|x 0
980 _ _ |a poster
980 _ _ |a VDB
980 _ _ |a I:(DE-Juel1)IEK-9-20110218
980 _ _ |a UNRESTRICTED
981 _ _ |a I:(DE-Juel1)IET-1-20110218


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