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@ARTICLE{Nazmutdinova:1020534,
      author       = {Nazmutdinova, Elina and Rosenbach, Carolin and Schmidt,
                      Christina and Sarawutankul, Sangchai and Neuhaus, Kerstin
                      and Gröschel, André and Vargas-Barbosa, Nella},
      title        = {{O}n the {I}nfluence of {L}i3{I}n{C}l6‐{PEDOT}:{PSS}
                      {H}ybrids in {S}olid‐{S}tate {B}atteries {P}repared via an
                      {A}queous {O}ne‐{P}ot {A}pproach},
      journal      = {Batteries $\&$ supercaps},
      volume       = {7},
      number       = {3},
      issn         = {2566-6223},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-00247},
      pages        = {e202300434},
      year         = {2024},
      abstract     = {Solid-state batteries (SSBs) utilizing halide solid
                      electro-lytes (SE) have garnered attention due to their
                      enhanced stability when paired with oxide-based cathode
                      active materials. However, the dynamic interparticle contact
                      during cycling in SSBs poses challenges to their stability
                      and performance. To mitigate this problem, in this study, we
                      present a one-pot, aqueous synthesis of composites that
                      integrate ion conductivity, electron conductivity, and
                      mechanical sta-bility into a single material. The developed
                      composites consist of a halide SE, lithium indium chloride
                      (Li3InCl6), and a conductive polymer (CP),
                      poly(3,4-ethylendioxythiophene)/poly(styrene sulfonate)
                      (PEDOT:PSS). The successful synthesis was verified using
                      spectroscopic, thermal, scattering, and microscopy methods,
                      with Kelvin Probe Force Microscopy (KPFM) demonstrating the
                      distribution of PEDOT:PSS at thegrain boundaries between
                      Li3InCl6particles. Upon incorporating our composite material
                      with lithium nickel manganese cobalt oxide (NMC) cathode
                      active material (CAM) as catholyte, an increase in the
                      partial electronic transport was observed with increasing CP
                      content. A direct correlation between the partial electronic
                      transport of the catholytes and the initial discharge
                      capacities was demonstrated. This study lays the groundwork
                      for the preparation of multi-functional catholytes under
                      more sustainable conditions, without the need for organic
                      solvents, extremely high temperatures, or special
                      environments},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1222 - Components and Cells (POF4-122) / 1223 - Batteries
                      in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1222 / G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001143231500001},
      doi          = {10.1002/batt.202300434},
      url          = {https://juser.fz-juelich.de/record/1020534},
}