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@ARTICLE{Gerhorst:1020565,
author = {Gerhorst, Christian-Roman and Neukirchen, Alexander and
Klüppelberg, Daniel A and Bihlmayer, Gustav and Betzinger,
Markus and Michalicek, Gregor and Wortmann, Daniel and
Blügel, Stefan},
title = {{P}honons from density-functional perturbation theory using
the all-electron full-potential linearized augmented
plane-wave method {FLEUR} *},
journal = {Electronic structure},
volume = {6},
number = {1},
issn = {2516-1075},
address = {Philadelphia, PA},
publisher = {IOP Publishing Ltd.},
reportid = {FZJ-2024-00260},
pages = {017001 -},
year = {2024},
abstract = {Phonons are quantized vibrations of a crystal lattice that
play a crucial role in understanding many properties of
solids. Density functional theory provides a
state-of-the-art computational approach to lattice
vibrations from first-principles. We present a successful
software implementation for calculating phonons in the
harmonic approximation, employing density-functional
perturbation theory within the framework of the
full-potential linearized augmented plane-wave method as
implemented in the electronic structure package FLEUR. The
implementation, which involves the Sternheimer equation for
the linear response of the wave function, charge density,
and potential with respect to infinitesimal atomic
displacements, as well as the setup of the dynamical matrix,
is presented and the specifics due to the muffin-tin sphere
centered linearized augmented plane-wavebasis-set and the
all-electron nature are discussed. As a test, we calculate
the phonon dispersion of several solids including an
insulator, a semiconductor as well as several metals. The
latter arecomprised of magnetic, simple, and transition
metals. The results are validated on the basis of phonon
dispersions calculated using the finite displacement
approach in conjunction with theFLEUR code and the phonopy
package, as well as by some experimental results. An
excellent agreement is obtained.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {621.3},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {5211 - Topological Matter (POF4-521) / MaX - MAterials
design at the eXascale. European Centre of Excellence in
materials modelling, simulations, and design (824143)},
pid = {G:(DE-HGF)POF4-5211 / G:(EU-Grant)824143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001136650200001},
doi = {10.1088/2516-1075/ad1614},
url = {https://juser.fz-juelich.de/record/1020565},
}