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| Hauptseite > Publikationsdatenbank > Sacrificial Catalyst of Carbothermal-Shock-Synthesized 1T-MoS2 Layers for Ultralong-Lifespan Seawater Battery > print |
| Hauptseite > Publikationsdatenbank > Sacrificial Catalyst of Carbothermal-Shock-Synthesized 1T-MoS2 Layers for Ultralong-Lifespan Seawater Battery > print |
| 001 | 1021218 | ||
| 005 | 20240712112831.0 | ||
| 024 | 7 | _ | |a 10.1021/acs.nanolett.2c04698 |2 doi |
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| 100 | 1 | _ | |a Son, Minjin |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Sacrificial Catalyst of Carbothermal-Shock-Synthesized 1T-MoS2 Layers for Ultralong-Lifespan Seawater Battery |
| 260 | _ | _ | |a Washington, DC |c 2023 |b ACS Publ. |
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| 520 | _ | _ | |a A Pt-nanoparticle-decorated 1T-MoS2 layer is designed as a sacrificial electrocatalyst by carbothermal shock (CTS) treatment to improve the energy efficiency and lifespan of seawater batteries. The phase transition of MoS2 crystals from 2H to metallic 1T─induced by the simple but potent CTS treatment─improves the oxygen-reduction-reaction (ORR) activity in seawater catholyte. In particular, the MoS2-based sacrificial catalyst effectively decreases the overpotential during charging via edge oxidation of MoS2, enhancing the cycling stability of the seawater battery. Furthermore, Pt nanoparticles are deposited onto CTS-MoS2 via an additional CTS treatment. The resulting specimen exhibits a significantly low charge/discharge potential gap of Δ0.39 V, high power density of 6.56 mW cm–2, and remarkable cycling stability up to ∼200 cycles (∼800 h). Thus, the novel strategy reported herein for the preparation of Pt-decorated 1T-MoS2 by CTS treatment could facilitate the development of efficient bifunctional electrocatalysts for fabricating seawater batteries with long service life. |
| 536 | _ | _ | |a 1223 - Batteries in Application (POF4-122) |0 G:(DE-HGF)POF4-1223 |c POF4-122 |f POF IV |x 0 |
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| 700 | 1 | _ | |a Park, Jaehyun |0 P:(DE-HGF)0 |b 1 |
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| 700 | 1 | _ | |a Ryu, Jong Hun |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Durmus, Yasin Emre |0 P:(DE-Juel1)162243 |b 4 |
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| 700 | 1 | _ | |a Kang, Seok Ju |0 P:(DE-HGF)0 |b 6 |e Corresponding author |
| 773 | _ | _ | |a 10.1021/acs.nanolett.2c04698 |g Vol. 23, no. 1, p. 344 - 352 |0 PERI:(DE-600)2048866-X |n 1 |p 344 - 352 |t Nano letters |v 23 |y 2023 |x 1530-6984 |
| 856 | 4 | _ | |y Published on 2022-12-27. Available in OpenAccess from 2023-12-27. |u https://juser.fz-juelich.de/record/1021218/files/Manuscirpt%20_for%20Nano%20Lett..pdf |
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