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@ARTICLE{SchulzeKppers:1021499,
author = {Schulze-Küppers, Falk and Duburg, Jacobus C. and Deibert,
Wendelin and Sohn, Yoo Jung and Guillon, Olivier and Sebold,
Doris and Natour, Ghaleb and Meulenberg, Wilhelm Albert},
title = {{I}nteraction between proton conducting
{B}a{C}e0.2{Z}r0.7{Y}0.1{O}3 electrolyte and structural
ceramics during sintering},
journal = {Journal of the European Ceramic Society},
volume = {44},
number = {5},
issn = {0955-2219},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2024-00792},
pages = {2762 - 2769},
year = {2024},
abstract = {The chemical compatibility of thin electrolyte layers and
their support materials at high temperatures is crucial for
the performance in solid oxide cells and membranes. This
work describes the chemical interaction between the
electrolyte material, BaCe0.2Zr0.7Y0.1O3 + 0.5 $wt\%$ NiO
(BCZY), and structural ceramics Al2O3, 8 $mol\%$
yttriastabilized zirconia (8YSZ), TiO2, CeO2 and MgO during
sintering. 1:1 $wt\%$ powder mixtures of the electrolyte
material and structural ceramics were annealed at 1500 ◦C
for 5 h, with the phase composition being determined through
XRD analysis at room temperature. Subsequently, the material
interaction between BCZY films depositedon the most
promising structural ceramic MgO was investigated by SEM and
EDS. In particular, the complex sintering requirements to
form single-phase BCZY electrolyte layers is troubled upon
coating and sintering BCZY on MgO. Hereby, the diffusion of
NiO into the MgO support leads to a deficiency of NiO in the
BCZY layer,making the solution and precipitation mechanism
required to form the perovskitic phase unable to occur. In
extreme scenarios, the electrolyte layer depletion of NiO
can even cause the decomposition of a single-phase BCZY into
BaZrO3, Ce-Y fluorite and a BCZY perovskite phase of
undefined composition.},
cin = {ZEA-1 / IEK-1 / JARA-ENERGY},
ddc = {660},
cid = {I:(DE-Juel1)ZEA-1-20090406 / I:(DE-Juel1)IEK-1-20101013 /
$I:(DE-82)080011_20140620$},
pnm = {1232 - Power-based Fuels and Chemicals (POF4-123) /
Verbundvorhaben PROMETHEUS2018: PROtonen und Sauerstoff
ko-ionische Leiter für CO2/H2O Ko-Elektrolyse und
Umwandlung zu METhanol und andere Chemikalien für ein
nachhaltiges EU-EnergieSystem (03SF0555A) / 1231 -
Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1232 / G:(BMBF)03SF0555A /
G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001168406000001},
doi = {10.1016/j.jeurceramsoc.2023.12.050},
url = {https://juser.fz-juelich.de/record/1021499},
}