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@ARTICLE{RochaOrtiz:1021595,
author = {Rocha-Ortiz, Juan S. and Wu, Jianchang and Wenzel, Jonas
and Bornschlegl, Andreas J. and Perea, Jose Dario and Leon,
Salvador and Barabash, Anastasia and Wollny, Anna-Sophie and
Guldi, Dirk M. and Zhang, Jiyun and Insuasty, Alberto and
Lüer, Larry and Ortiz, Alejandro and Hirsch, Andreas and
Brabec, Christoph},
title = {{E}nhancing {P}lanar {I}nverted {P}erovskite {S}olar
{C}ells with {I}nnovative {D}umbbell‐{S}haped {HTM}s: {A}
{S}tudy of {H}exabenzocoronene and
{P}yrene‐{BODIPY}‐{T}riarylamine {D}erivatives},
journal = {Advanced functional materials},
volume = {33},
number = {44},
issn = {1616-301X},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2024-00858},
pages = {2304262},
year = {2023},
abstract = {Dumbbell-shaped systems based on PAHs-BODIPY-triarylamine
hybrids TM-(01-04) are designed as novel and highly
efficient hole-transporting materials for usage in planar
inverted perovskite solar cells. BODIPY is employed as a
bridge between the PAH units, and the effects of the
conjugated π-system's covalent attachment and size are
investigated. Fluorescence quenching, 3D fluorescence heat
maps, and theoretical studies support energy transfer within
the moieties. The systems are extremely resistant to UVC 254
nm germicidal light sources and present remarkable thermal
stability at degradation temperatures exceeding 350 °C.
Integrating these systems into perovskite solar cells
results in outstanding power conversion efficiency (PCE),
with TM-02-based devices exhibiting a PCE of $20.26\%.$ The
devices base on TM-01, TM-03, and TM-04 achieve PCE values
of $16.98\%,$ $17.58\%,$ and $18.80\%,$ respectively. The
long-term stability of these devices is measured for 600 h,
with initial efficiency retention between $94\%$ and $86\%.$
The TM-04-based device presents noticeable stability of
$94\%,$ better than the reference polymer PTAA with $91\%.$
These findings highlight the exciting potential of
dumbbell-shaped systems based on PAHs-BODIPY-triarylamine
derivatives for next-generation photovoltaics.},
cin = {IEK-11},
ddc = {530},
cid = {I:(DE-Juel1)IEK-11-20140314},
pnm = {1213 - Cell Design and Development (POF4-121)},
pid = {G:(DE-HGF)POF4-1213},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001024900700001},
doi = {10.1002/adfm.202304262},
url = {https://juser.fz-juelich.de/record/1021595},
}