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@INPROCEEDINGS{Reinecke:1022271,
author = {Reinecke, Ernst-Arndt and Nobrega, Gabriela and Klauck,
Michael},
title = {{E}xperiments on the impact of carbon monoxide on the
efficiency of catalysts used for hydrogen mitigation in the
late phase of a severe accident},
reportid = {FZJ-2024-01389},
year = {2023},
abstract = {The molten core-concrete interaction in the ex-vessel phase
of a severe accident in a light water reactor is the source
of significant amounts of carbon monoxide among other
gaseous products. The European project AMHYCO addresses open
issues related to the understanding of the impact of carbon
monoxide on phenomena occurring in the late accident phase.
One of these topics is related to the impact on the
operational behavior of passive auto-catalytic recombiners
(PARs). An experimental program alongside model development
activities aims to improve the predictive capabilities of
numerical models in order to assess the efficiency of PARs
as hydrogen mitigation measure.Experiments in the REKO-3
facility are being performed to study the impact of carbon
monoxide on both platinum-based and palladium-based
catalysts. Catalyst sheets are exposed to steady-state flows
of gaseous mixtures including hydrogen, oxygen, nitrogen,
steam and carbon monoxide inside a vertical flow reactor.
The boundary conditions are selected according to numerical
pre-studies in order to cover relevant ranges of gaseous
mixtures. Specific focus lies on mixtures with low amounts
of oxygen. Measurements of the catalyst temperature and the
outlet gas concentrations enable to assess the catalyst
activity and efficiency.The conference paper gives a
comprehensive overview of the work performed, introduces the
experimental facility, and highlights relevant
results.KEYWORDSSevere Accident, Hydrogen Mitigation,
Passive Auto catalytic Recombiners, Carbon Monoxide},
month = {Aug},
date = {2023-08-20},
organization = {20th International Topical Meeting on
Nuclear Reactor Thermal Hydraulics
(NURETH-20), Washington (USA), 20 Aug
2023 - 25 Aug 2023},
cin = {IEK-14},
cid = {I:(DE-Juel1)IEK-14-20191129},
pnm = {1422 - Beyond Design Basis Accidents and Emergency
Management (POF4-142)},
pid = {G:(DE-HGF)POF4-1422},
typ = {PUB:(DE-HGF)1},
url = {https://juser.fz-juelich.de/record/1022271},
}