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@ARTICLE{Bela:1024077,
      author       = {Bela, Marlena M. and Schmidt, Christina and Neuhaus,
                      Kerstin and Hering, Tobias and Stan, Marian C. and Winter,
                      Martin and Börner, Markus},
      title        = {{T}unable {L}i{Z}n‐{I}ntermetallic {C}oating {T}hickness
                      on {L}ithium {M}etal and {I}ts {E}ffect on {M}orphology and
                      {P}erformance in {L}ithium {M}etal {B}atteries},
      journal      = {Advanced materials interfaces},
      volume       = {11},
      number       = {13},
      issn         = {2196-7350},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-01957},
      pages        = {2300836},
      year         = {2024},
      abstract     = {Lithium metal batteries are promising next-generation
                      rechargeable batteries with high energy density. However,
                      the high reactivity of lithium metal leads to an undesirable
                      growth of high surface area lithium during electrodeposition
                      and -dissolution and remains a key challenge that must be
                      addressed to enable commercialization. Modification of the
                      Li metal surface to obtain protective coatings is a common
                      method to overcome these challenges. In this study, the
                      influence of the thickness of an intermetallic coating on Li
                      metal is investigated after application by means of thermal
                      evaporation. In addition, the relevance of pre-treatments in
                      reducing the native layer thickness and surface roughness by
                      roll-pressing Li metal prior to coating is demonstrated.
                      Morphological analyses are performed on cross-sections
                      prepared under cryogenic conditions to investigate the
                      origin of high surface area lithium growth and coating
                      cracks after electrodeposition and -dissolution processes.
                      The results obtained support the conclusion that the
                      exclusive combination of roll-pressed Li metal foil followed
                      by coating reduces overvoltage and improves cycle life at
                      elevated current densities.},
      cin          = {IEK-12},
      ddc          = {600},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1212 - Materials and Interfaces (POF4-121) / 1213 - Cell
                      Design and Development (POF4-121)},
      pid          = {G:(DE-HGF)POF4-1212 / G:(DE-HGF)POF4-1213},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001184616000001},
      doi          = {10.1002/admi.202300836},
      url          = {https://juser.fz-juelich.de/record/1024077},
}