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@ARTICLE{Miao:1024256,
author = {Miao, H. and Bouaziz, Juba and Fabbris, G. and Meier, W. R.
and Yang, F. Z. and Li, H. X. and Nelson, C. and Vescovo, E.
and Zhang, S. and Christianson, A. D. and Lee, H. N. and
Zhang, Y. and Batista, C. D. and Blügel, S.},
title = {{S}pontaneous {C}hirality {F}lipping in an {O}rthogonal
{S}pin-{C}harge {O}rdered {T}opological {M}agnet},
journal = {Physical review / X},
volume = {14},
number = {1},
issn = {2160-3308},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2024-02063},
pages = {011053},
year = {2024},
abstract = {The asymmetric distribution of chiral objects with opposite
chirality is of great fundamental interest ranging from
molecular biology to particle physics. In quantum materials,
chiral states can build on inversion-symmetry-breaking
lattice structures or emerge from spontaneous magnetic
ordering induced by competing interactions. Although the
handedness of a chiral state can be changed through external
fields, a spontaneous chirality flipping has yet to be
discovered. We present experimental evidence of chirality
flipping via changing temperature in a topological magnet
EuAl4, which features orthogonal spin density waves (SDW)
and charge density waves (CDW). Using circular dichroism of
Bragg peaks in the resonant magnetic x-ray scattering, we
find that the chirality of the helical SDW flips through a
first-order phase transition with modified SDW wavelength.
Intriguingly, we observe that the CDW couples strongly with
the SDW and displays a rare commensurate-to-incommensurate
transition at the chirality flipping temperature. Combining
with first-principles calculations and angle-resolved
photoemission spectroscopy, our results support a Fermi
surface origin of the helical SDW with intertwined spin,
charge, and lattice degrees of freedom in EuAl4. Our results
reveal an unprecedented spontaneous chirality flipping and
lay the groundwork for a new functional manipulation of
chirality through momentum-dependent spin-charge-lattice
interactions.},
cin = {PGI-1},
ddc = {530},
cid = {I:(DE-Juel1)PGI-1-20110106},
pnm = {5211 - Topological Matter (POF4-521) / 3D MAGiC -
Three-dimensional magnetization textures: Discovery and
control on the nanoscale (856538) / SFB 1238 C01 -
Strukturinversionsasymmetrische Materie und
Spin-Orbit-Phänomene mittels ab initio (C01) (319898210) /
DFG project 403503315 - Grenzflächenstabilisierte
Skyrmionen in Oxidstrukturen für die Skyrmionik
(403503315)},
pid = {G:(DE-HGF)POF4-5211 / G:(EU-Grant)856538 /
G:(GEPRIS)319898210 / G:(GEPRIS)403503315},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001195847000002},
doi = {10.1103/PhysRevX.14.011053},
url = {https://juser.fz-juelich.de/record/1024256},
}