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@ARTICLE{Ye:1024445,
      author       = {Ye, Ruijie and Hamzelui, Niloofar and Ihrig, Martin and
                      Finsterbusch, Martin and Figgemeier, Egbert},
      title        = {{W}ater-{B}ased {F}abrication of a
                      {L}i|{L}i7{L}a3{Z}r2{O}12 |{L}i{F}e{PO}4 {S}olid-{S}tate
                      {B}attery─{T}oward {G}reen {B}attery {P}roduction},
      journal      = {ACS sustainable chemistry $\&$ engineering},
      volume       = {10},
      number       = {23},
      issn         = {2168-0485},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {FZJ-2024-02188},
      pages        = {7613 - 7624},
      year         = {2022},
      abstract     = {Solid-state lithium batteries (SSLBs) are considered to be
                      one of the most promising next-generation Li batteries due
                      to their high capacity and intrinsic safety. However, their
                      sustainable processing is often poorly investigated but
                      could offer additional advantages over conventional
                      batteries in terms of ecological and economic benefits. In
                      this work, a sustainable, water-based processing route for
                      garnet-supported SSLBs featuring a LiFePO4
                      (LFP)-poly(ethylene oxide) (PEO) composite cathode is
                      presented. Both the LFP-PEO cathode and the thin
                      free-standing garnet separator (105 μm) are fabricated by
                      water-based tape-casting. After optimizing the composition
                      of the cathode, the full cell with a thin cathode (∼45
                      μm) delivers a high capacity of 136 mAh g–1 with a high
                      Coulombic efficiency over $99\%$ and good cycling stability
                      for 50 cycles. However, the performance and cycling
                      stability decrease when thicker cathodes (∼110 μm) and
                      higher rates were applied, indicating the need for further
                      optimization. Nevertheless, the here-presented water-based
                      fabrication route provides a baseline for further
                      improvements and pushes SSLB fabrication further toward a
                      green battery production.},
      cin          = {IEK-1 / IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000813628900001},
      doi          = {10.1021/acssuschemeng.2c01349},
      url          = {https://juser.fz-juelich.de/record/1024445},
}