001024677 001__ 1024677
001024677 005__ 20250204113826.0
001024677 0247_ $$2doi$$a10.1016/j.jpowsour.2024.234394
001024677 0247_ $$2ISSN$$a0378-7753
001024677 0247_ $$2ISSN$$a1873-2755
001024677 0247_ $$2datacite_doi$$a10.34734/FZJ-2024-02350
001024677 0247_ $$2WOS$$aWOS:001218339700001
001024677 037__ $$aFZJ-2024-02350
001024677 082__ $$a620
001024677 1001_ $$0P:(DE-HGF)0$$aWang, Chih-Chieh$$b0$$eCorresponding author
001024677 245__ $$aGrain boundary complexion modification for interface stability in garnet based solid-state Li batteries
001024677 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2024
001024677 3367_ $$2DRIVER$$aarticle
001024677 3367_ $$2DataCite$$aOutput Types/Journal article
001024677 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1713364749_6813
001024677 3367_ $$2BibTeX$$aARTICLE
001024677 3367_ $$2ORCID$$aJOURNAL_ARTICLE
001024677 3367_ $$00$$2EndNote$$aJournal Article
001024677 520__ $$aThe garnet type solid-state electrolyte (SSE) encounters challenges related to poor interfacial contact with Li metal and dendrite penetration problem. This study addresses these issues by manipulating the surface property of garnet-based LLZTO (Li6.5La3Zr1.6Ta0.4O12) SSE. The manipulation is achieved by varying thickness of Al2O3 atomic layer deposition (ALD), followed by sintering. Research results show that the relative density, ionic conductivity, and hardness of LLZTO are improved while electronic conductivity is reduced due to the formation of multiple complexions at grain boundary (GB). The SSE pellets also demonstrate improved wettability with Li metal, leading to stable galvanostatic Li plating/stripping cycling with low polarization, which allows for batter battery performance than pristine one. The concept of modifying SSE through the grain boundary complexion modification by thin ALD coating for enhancing the dendrite tolerance with better electrochemical properties of SSE may open a new direction for solid state battery research.
001024677 536__ $$0G:(DE-HGF)POF4-1223$$a1223 - Batteries in Application (POF4-122)$$cPOF4-122$$fPOF IV$$x0
001024677 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
001024677 7001_ $$0P:(DE-HGF)0$$aHsu, Wei-Chun$$b1
001024677 7001_ $$0P:(DE-HGF)0$$aChang, Chia-Yu$$b2
001024677 7001_ $$0P:(DE-Juel1)174298$$aIhrig, Martin$$b3
001024677 7001_ $$0P:(DE-HGF)0$$aThuy Tran, Ngoc Thanh$$b4
001024677 7001_ $$0P:(DE-HGF)0$$aLin, Shih-kang$$b5
001024677 7001_ $$0P:(DE-Juel1)188297$$aWindmüller, Anna$$b6
001024677 7001_ $$0P:(DE-Juel1)156244$$aTsai, Chih-Long$$b7
001024677 7001_ $$0P:(DE-Juel1)156123$$aEichel, Rüdiger-A.$$b8$$ufzj
001024677 7001_ $$0P:(DE-HGF)0$$aChiu, Kuo-Feng$$b9
001024677 773__ $$0PERI:(DE-600)1491915-1$$a10.1016/j.jpowsour.2024.234394$$gVol. 602, p. 234394 -$$p234394 -$$tJournal of power sources$$v602$$x0378-7753$$y2024
001024677 8564_ $$uhttps://doi.org/10.1016/j.jpowsour.2024.234394
001024677 8564_ $$uhttps://juser.fz-juelich.de/record/1024677/files/SSE-LLZO-ALD-20231012-FINAL-Long.docx$$yPublished on 2024-03-23. Available in OpenAccess from 2026-03-23.
001024677 8564_ $$uhttps://juser.fz-juelich.de/record/1024677/files/Supporting%20information-20231012-FINAL-Long.docx$$yPublished on 2024-03-23. Available in OpenAccess from 2026-03-23.
001024677 909CO $$ooai:juser.fz-juelich.de:1024677$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
001024677 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)188297$$aForschungszentrum Jülich$$b6$$kFZJ
001024677 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156244$$aForschungszentrum Jülich$$b7$$kFZJ
001024677 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156123$$aForschungszentrum Jülich$$b8$$kFZJ
001024677 9101_ $$0I:(DE-588b)36225-6$$6P:(DE-Juel1)156123$$aRWTH Aachen$$b8$$kRWTH
001024677 9131_ $$0G:(DE-HGF)POF4-122$$1G:(DE-HGF)POF4-120$$2G:(DE-HGF)POF4-100$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-1223$$aDE-HGF$$bForschungsbereich Energie$$lMaterialien und Technologien für die Energiewende (MTET)$$vElektrochemische Energiespeicherung$$x0
001024677 9141_ $$y2024
001024677 915__ $$0LIC:(DE-HGF)CCBYNCND4$$2HGFVOC$$aCreative Commons Attribution-NonCommercial-NoDerivs CC BY-NC-ND 4.0
001024677 915__ $$0StatID:(DE-HGF)0530$$2StatID$$aEmbargoed OpenAccess
001024677 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2023-08-28
001024677 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2023-08-28
001024677 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bJ POWER SOURCES : 2022$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2024-12-06
001024677 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bJ POWER SOURCES : 2022$$d2024-12-06
001024677 920__ $$lyes
001024677 9201_ $$0I:(DE-Juel1)IEK-9-20110218$$kIEK-9$$lGrundlagen der Elektrochemie$$x0
001024677 9801_ $$aFullTexts
001024677 980__ $$ajournal
001024677 980__ $$aVDB
001024677 980__ $$aUNRESTRICTED
001024677 980__ $$aI:(DE-Juel1)IEK-9-20110218
001024677 981__ $$aI:(DE-Juel1)IET-1-20110218