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@ARTICLE{Zhang:1024683,
      author       = {Zhang, Heng and Qiao, Lixin and Kühnle, Hannes and
                      Figgemeier, Egbert and Armand, Michel and Eshetu, Gebrekidan
                      Gebresilassie},
      title        = {{F}rom lithium to emerging mono- and
                      multivalent-cation-based rechargeable batteries: non-aqueous
                      organic electrolyte and interphase perspectives},
      journal      = {Energy $\&$ environmental science},
      volume       = {16},
      number       = {1},
      issn         = {1754-5692},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {FZJ-2024-02356},
      pages        = {11 - 52},
      year         = {2023},
      abstract     = {Since the oil crisis in the 1970s, the importance of
                      rechargeable batteries has been noted by both academia and
                      industry. This has become more prominent with the increasing
                      demand in e-mobility and integration of renewable sources in
                      the energy ecosystem. However, despite the great success of
                      lithium-ion batteries in portable consumer electronics and
                      the above-mentioned domains, it is challenging to further
                      expand their use to large-volume technical applications due
                      to the limited resources of some key elements (lithium,
                      cobalt, etc.). Accordingly, emerging mono-valent (e.g.,
                      sodium and potassium) and multi-valent (magnesium, calcium,
                      zinc, aluminum, etc.) batteries are expected to overcome the
                      resource limitation and related challenges. Herein, we
                      present the historical development of non-aqueous organic
                      electrolytes and electrode–electrolyte interphases and
                      focus on the similarities and differences between
                      lithium-based batteries and other complementary emerging
                      battery technologies. Special attention is paid to some
                      basic parameters related to solvents and salts, including
                      donor numbers and Eigen values, to better understand the
                      transport behavior in the bulk electrolyte. Moreover, key
                      parameters impacting the features of the
                      electrode–electrolyte interphase are critically analyzed
                      for each battery configuration. Additionally, we discuss the
                      possible strategies to enhance the physical (e.g., transport
                      behavior and mechanical properties) and (electro)chemical
                      properties of electrolytes and interphases, aiming at
                      promoting the development of sustainable and
                      high-performance mono- and multi-valent batteries for
                      practical applications. Particularly, it is scrutinized
                      whether the accumulated facts with respect to lithium can be
                      smoothly transferred to other emerging battery systems or
                      not.},
      cin          = {IEK-12},
      ddc          = {690},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000892830100001},
      doi          = {10.1039/D2EE02998G},
      url          = {https://juser.fz-juelich.de/record/1024683},
}