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@ARTICLE{Pirona:1024691,
author = {Pirona, Lorenza and Ballabio, Federico and Alfonso-Prieto,
Mercedes and Capelli, Riccardo},
title = {{C}alcium-driven {I}n {S}ilico {I}nactivation of a {H}uman
{O}lfactory {R}eceptor},
journal = {bioRxiv beta},
address = {Cold Spring Harbor},
publisher = {Cold Spring Harbor Laboratory, NY},
reportid = {FZJ-2024-02364},
year = {2024},
note = {Preprint publicly available; peer-reviewed version was
published in Journal of Chemical Information and Modeling
(doi: 10.1021/acs.jcim.4c00249)},
abstract = {Conformational changes as well as molecular determinants
related to the activation and inactivation of olfactory
receptors are still poorly understood due to the intrinsic
difficulties in the structural determination of this GPCR
family. Here, we perform, for the first time, the in silico
inactivation of the human olfactory receptor OR51E2,
highlighting the possible role of calcium in this receptor
state transition. Using molecular dynamics simulations, we
show that a divalent ion in the ion binding site,
coordinated by two acidic residues at positions 2.50 and
3.39 conserved across most ORs, stabilizes the receptor in
its inactive state. In contrast, protonation of the same two
acidic residues is not sufficient to drive inactivation
within the µs timescale of our simulations. Our findings
suggest a novel molecular mechanism for OR inactivation,
potentially guiding experimental validation and offering
insights into the possible broader role of divalent ions in
GPCR signaling.},
cin = {IAS-5 / INM-9},
ddc = {570},
cid = {I:(DE-Juel1)IAS-5-20120330 / I:(DE-Juel1)INM-9-20140121},
pnm = {5241 - Molecular Information Processing in Cellular Systems
(POF4-524) / DFG project 291198853 - FOR 2518: Funktionale
Dynamik von Ionenkanälen und Transportern - DynIon -
(291198853) / DFG project 329460521 - Protonentransfer und
Substraterkennung in SLC17-Transportern (329460521)},
pid = {G:(DE-HGF)POF4-5241 / G:(GEPRIS)291198853 /
G:(GEPRIS)329460521},
typ = {PUB:(DE-HGF)25},
doi = {10.1101/2024.01.31.578070},
url = {https://juser.fz-juelich.de/record/1024691},
}